Control of fragmentation reactions in impulsively aligned polyatomic molecules by selective removal of inner-valence electrons

机译：通过选择性去除内价电子来控制脉冲排列的多原子分子中的断裂反应

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Recently, selective fragmentation of polyatomic molecules using the carrier-envelope phase (CEP) of few-cycle ionizing laser pulses as the control parameter [1] has been demonstrated [2]. It was shown that the underlying mechanism is selective removal of specific (inner-valence shell) electrons, which puts the molecule into a dedicated dissociative electronic state from which the molecule then fragments along a desired pathway.

机译：近来，已经证明了使用几个周期的电离激光脉冲的载流子包络相（CEP）作为控制参数[1]来选择性分裂多原子分子[2]。结果表明，潜在的机理是选择性去除特定的（内价壳层）电子，这使分子进入专用的解离电子状态，然后分子从该状态开始沿着所需的路径断裂。

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《2013 Conference on Lasers and Electro-Optics Europe amp; International Quantum Electronics Conference》|2013年|1|共1页
会议地点 Munich(DE)
作者
Xie X.; Doblhoff-Dier K.; Xu H.; Roither S.;
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Photonics Institute, Vienna University of Technology, Vienna, Austriac;

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正文语种 eng
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专利

1. Selective Control over Fragmentation Reactions in Polyatomic Molecules Using Impulsive Laser Alignment [J] . Xinhua Xie, Katharina Doblhoff-Dier, Huailiang Xu, Physical review letters . 2014,第16期

机译：脉冲激光对准对多原子分子裂解反应的选择性控制
2. Attosecond-Recollision-Controlled Selective Fragmentation of Polyatomic Molecules [J] . Xinhua Xie, Katharina Doblhoff-Dier, Stefan Roither, Physical review letters . 2012,第24期

机译：阿托秒碰撞控制的多原子分子选择性裂解
3. Theory and Control of Thermal Photoinduced Electron Transfer Reactions in Polyatomic Molecules [J] . Eli Pollak, Yong He The journal of physical chemistry, B. Condensed matter, materials, surfaces, interfaces & biophysical . 2001,第28期

机译：多原子分子中热光诱导电子转移反应的理论与控制
4. Control of fragmentation reactions in impulsively aligned polyatomic molecules by selective removal of inner-valence electrons [C] . Xie X., Doblhoff-Dier K., Xu H., 2013 Conference on Lasers and Electro-Optics Europe Internationaluantum Electronics Conference . 2013

机译：通过选择性移除内值电子的脉冲对齐的多原子分子在脉冲对齐的多原子分子中的控制
5. Energy partitioning in polyatomic chemical reactions: Quantum state resolved studies of highly exothermic atom abstraction reactions from molecules in the gas phase and at the gas-liquid interface. [D] . Zolot, Alexander M. 2009

机译：多原子化学反应中的能量分配：量子态分解研究，涉及气相和气液界面中分子的高度放热原子提取反应。
6. Reconstruction of two-dimensional molecular structure with laser-induced electron diffraction from laser-aligned polyatomic molecules [O] . Chao Yu, Hui Wei, Xu Wang, -1

机译：激光取向的多原子分子的激光诱导电子衍射重建二维分子结构
7. Selective Control over Fragmentation Reactions in Polyatomic Molecules Using Impulsive Laser Alignment [O] . Xinhua Xie, Katharina Doblhoff-Dier, Huailiang Xu, 2014

机译：使用脉冲激光对准选择性控制多原子分子中的碎片反应

Control of fragmentation reactions in impulsively aligned polyatomic molecules by selective removal of inner-valence electrons

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