Control over two-dimensional vibrational trajectory by phase-shaped infrared pulses

机译：通过相位形红外脉冲控制二维振动轨迹

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We demonstrate that relative phase between two vibrational excitations in a metal di-carbonyl compound was controlled by phase-shaped mid-infrared pulses. The control over the relative phase between two normal modes of symmetric and anti-symmetric carbonyl stretch modes corresponds to control over two-dimensional vibrational trajectory at the initial stage after excitation.

机译：我们证明了在金属二羰基化合物中的两个振动激发之间的相对相位是由相形的中红外脉冲控制的。对对称和反对称羰基拉伸模式的两个正常模式之间的相对相位的控制对应于在激发之后的初始阶段对二维振动轨迹的控制。

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《CLEO;Conference on Lasers and Electro-Optics》|2012年|p.1- 2|共2页
会议地点 San Jose, CA(US)
作者
Ashihara, Satoshi;
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Dept. of Applied Physics Tokyo Univ. of Agriculture and Technology 2-24-16 Nakacho Koganei Tokyo 184-8588 Japan;

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2. Controlling condensed-phase vibrational excitation with tailored infrared pulses [J] . V. D. Kleiman, S. M. Arrivo, J. S. Melinger, Chemical Physics: A Journal Devoted to Experimental and Theoretical Research Involving Problems of Both a Chemical and Physical Nature . 1998,第2a3期

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3. CONTROLLED SURFACE PHOTOCHEMISTRY - BOND- AND ISOTOPE-SELECTIVE PHOTODESORPTION OF NEUTRALS BY ADSORBATE VIBRATIONAL PREPARATION WITH INFRARED LASER PULSES [J] . Saalfrank P., Paramonov GK. The Journal of Chemical Physics . 1997,第24期

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4. Control over Two-dimensional Vibrational Trajectory by Phase-shaped Infrared Pulses [C] . Satoshi Ashihara, Kaori Enomoto, Toshiya Arakaki Conference on Lasers and Electro-Optics . 2012

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5. Two-Dimensional Infrared Vibrational Echo Spectroscopy Measurements of the Structural Dynamics Occurring in Conducting Polymer Thin Films [D] . Eigner, Audrey Ann 2011

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6. Two-dimensional infrared spectroscopy of peptides by phase-controlled femtosecond vibrational photon echoes [O] . M. C. Asplund, M. T. Zanni, R. M. Hochstrasser 2000

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Control over two-dimensional vibrational trajectory by phase-shaped infrared pulses

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