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DETERMINATION OF ~(238)Pu AND ~(239+240)Pu BY DESTRUCTIVE ASSAYS

机译:破坏性测定法测定〜(238)Pu和〜(239 + 240)Pu

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摘要

Analysis of plutonium in environmental samples is one of the measures recently included in international safeguards. Plutonium and some other actinides, and fission and activation products in environmental samples, are currently used as indications of undeclared nuclear activities. Two destructive assays are presented for determination of ~(238)Pu and ~(239+240)Pu in environmental samples. Alpha spectrometers were utilized to identify the isotopic composition of plutonium. The results show coincidence of the determined plutonium concentrations with certified values. The U test was used as a quality control indicator of the presented procedures and results. The levels of ~(238)Pu and ~(239+240)Pu in the samples ranged from 1.6 x 10~7 to 4.2 x 10~8 atoms, and from 2.2 x 10~(10) to 2.6 x 10~(11) atoms, respectively. Both methods could be applied for accurate, low level analysis to indicate plutonium origin.
机译:分析环境样品中的is是国际保障措施中最近包括的措施之一。 used和一些其他act系元素,以及环境样品中的裂变和活化产物,目前被用作未申报核活动的迹象。提出了两种破坏性测定法,用于测定环境样品中的〜(238)Pu和〜(239 + 240)Pu。利用α光谱仪鉴定p的同位素组成。结果表明确定的concentrations浓度与标准值一致。 U检验用作所提出程序和结果的质量控制指标。样品中〜(238)Pu和〜(239 + 240)Pu的水平范围为1.6 x 10〜7到4.2 x 10〜8个原子,以及2.2 x 10〜(10)到2.6 x 10〜(11) )原子。两种方法均可用于准确的低含量分析,以表明indicate的来源。

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