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Coupling of Geochemical Reactions and Convective Mixing in the Long-TermGeological Storage of Carbon Dioxide

机译:二氧化碳长期地质封存中地球化学反应与对流混合的耦合

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The effect of coupling of geochemical reactions with convective mixing of dissolved carbon dioxide during geological storage is investigated by both analytical and numerical techniques. In the limit of fast reactions, scaling arguments and stability analysis show that the time for the onset of convection could be increased by up to an order of magnitude due to consumption of the dissolved CO_2 in mineralization. Numerical simulations are then used to investigate the effect of general reaction rates in two contrasting mineralogies, including overall CO_2 dissolution and the distribution of ion and mineral concentrations.
机译:通过分析和数值技术研究了地质化学反应与溶解二氧化碳的对流混合耦合的影响。在快速反应的范围内,定标论证和稳定性分析表明,由于矿化过程中溶解的CO_2的消耗,对流开始的时间最多可以增加一个数量级。然后使用数值模拟研究了两种相反矿物学中一般反应速率的影响,包括总体CO_2溶解以及离子和矿物浓度的分布。

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