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Characteristics and correlations between size-segregated PAHs and carbonaceous component in aerosol in Beijing, China

机译:北京地区气溶胶中颗粒物中PAHs与碳组分的特征及相关性

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@@ 1.Introduction The carbonaceous material constitutes a significant component of total aerosol mass and it is composed by two main fractions, organic carbon (OC) and elemental carbon (EC). OC is a mixture of hydrocarbons and oxygenates, which can be directly emitted from sources (primary OC) or produced from atmospheric reactions involving gaseous organic precursors (secondary OC) (Pandis et al, 1992; Turpin and Huntzicker, 1995). With a chemical structure similar to impure graphite, generally EC is generated by the combustion of carbon-containing fuels. EC may not only intervene in some important chemical reactions in the atmosphere (Gundel et al., 1989) but also play an important role in global climate change by affecting radiative forcing and be the second most important component of global warming, after CO2 (Hansen et al, 2000; Jacobson, 2001). Menon et al. (2002) reported that over the past decades in China, the increased rainfall in the south and drought in the north might be related to the increased EC aerosol.Beijing, with an area of 16,807 km2 and a population over 16.3 million, is the economic, politics and culture center of China. Despite the evident significance of OC, EC and PAHs in atmospheric environmental process and human health, the study on their concentrations, sources and size distribution is quite poor in Beijing.
机译:@ 1.简介碳质材料是总气溶胶质量的重要组成部分,它由两个主要部分组成,有机碳(OC)和元素碳(EC)。 OC是碳氢化合物和含氧化合物的混合物,可以直接从源中排放(一次OC),也可以从涉及气态有机前体的大气反应中产生(二次OC)(Pandis等,1992; Turpin和Huntzicker,1995)。具有类似于不纯石墨的化学结构,通常EC是通过含碳燃料的燃烧产生的。 EC不仅可能干预大气中的一些重要化学反应(Gundel等,1989),而且还通过影响辐射强迫在全球气候变化中发挥重要作用,并且是仅次于CO2的全球变暖的第二重要组成部分(Hansen)等人,2000; Jacobson,2001)。 Menon等。 (2002年)报告说,在过去的几十年中,中国南部降雨的增加和北部干旱的发生可能与EC气溶胶的增加有关。北京经济面积16807平方公里,人口超过1630万。 ,中国政治文化中心。尽管OC,EC和PAH在大气环境过程和人类健康中具有明显的意义,但对它们的浓度,来源和大小分布的研究在北京还是很差的。

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