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Surface Patterning with SERS-Active Nanoparticle Aggregates for Safeguards Applications

机译:具有SERS活性纳米颗粒聚集体的表面图案,可用于保障应用

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In this paper, we describe our efforts to use spectroscopic signatures of materials to develop a passive tagging and sealing technology for safeguards applications. With spectroscopic responses defined by SANAs (SERS-Active Nanoparticle Aggregates; SERS: Surface-Enhanced Raman Scattering), we offer a potential robust, in-field verifiable barcoding capability with inexpensive materials. At INMM 2010, we showed SANA materials having improved robustness and spectral quality over older but similar materials, and we demonstrated how those materials might be combined with tags under development at Sandia National Laboratories (SNL). The SANA materials represent a component technology that might be implemented in a number of ways. Here, we will focus on our recent NGSI (Next Generation Safeguards Initiative) application development work involving small area surface deposition. With commercially available instrumentation, we are able to 'write' barcodes defined by both spatial properties and spectral responses into square millimeter areas for later readback using Raman mapping. We will describe our results with emphasis on integration of this technology into safeguards applications.
机译:在本文中,我们描述了我们使用材料的光谱特征来开发用于保障应用的无源标签和密封技术的努力。利用SANA(SERS-活性纳米粒子聚集体; SERS:表面增强拉曼散射)定义的光谱响应,我们可以提供廉价的材料,具有强大的,可现场验证的条码功能。在INMM 2010上,我们展示了SANA材料比旧的但相似的材料具有更高的鲁棒性和光谱质量,并且展示了这些材料如何与桑迪亚国家实验室(SNL)正在开发的标签结合使用。 SANA材料代表可以通过多种方式实施的组件技术。在这里,我们将重点关注涉及小面积表面沉积的最新NGSI(下一代保障措施)应用程序开发工作。利用市售的仪器,我们能够将由空间特性和光谱响应定义的条形码“写入”平方毫米区域,以便以后使用拉曼映射回读。我们将重点介绍将此技术集成到保障应用程序中来描述我们的结果。

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