A Less-Explored Surface Property: The Electrical Double Layer and Its Molecular Interrogation Capability

机译：较少开发的表面性质：电双层及其分子询问能力

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Exploiting the interfacial EDL structure as an analytical means to interrogate ionic and molecular properties is a groundbreaking shift in paradigm for molecular interrogation. In demonstrating the functionality of this new method, subtle changes in Cerium Oxide nanoparticles due to exposure to different redox environment was captured. This direct molecular interrogation using a simple EDL nanopore device will be a clear departure from the conventional bioanalytic techniques. Because intermediate molecules will be unnecessary, interaction between analyte targets and electrode surfaces can be dynamic and reversible as well as static and irreversible, and the sensing surface will be rugged with long functionality and shelf life.

机译：利用界面EDL结构作为质询离子和分子性质的分析手段，是分子审问范式的突破性转变。在演示此新方法的功能时，捕获了由于暴露于不同氧化还原环境而导致的氧化铈纳米颗粒的细微变化。使用简单的EDL纳米孔装置进行的直接分子询问将明显偏离传统的生物分析技术。由于不需要中间分子，因此分析物目标和电极表面之间的相互作用可以是动态和可逆的，也可以是静态和不可逆的，并且传感表面将坚固耐用，并具有较长的功能性和保质期。

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《Society for Biomaterials annual meeting and exposition》|2019年|351-351|共1页
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Yu Zhao; Sam Bearden; Guigen Zhang;
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1. Molecular dynamics simulations of the electrical double layer on smectite surfaces contacting concentrated mixed electrolyte (NaCl-CaCl_2) solutions [J] . Bourg I.C., Sposito G. Journal of Colloid and Interface Science . 2011,第2期

机译：蒙脱石表面与浓混合电解质（NaCl-CaCl_2）溶液接触的双电层的分子动力学模拟
2. Electrical, optical and surface properties of P_2S_5/(NH_4)_2S_x+Se-treated doped-channel field-effect transistors with double etch-stop layers [J] . Y.S. Lin, Y.T. Lin, Y.W. Huang Thin Solid Films . 2011,第10期

机译：具有双蚀刻终止层的P_2S_5 /（NH_4）_2S_x + Se处理的掺杂沟道场效应晶体管的电，光学和表面特性
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机译：十六烷基三甲基氯化铵水溶液的双电层性质
4. A Less-Explored Surface Property: The Electrical Double Layer and Its Molecular Interrogation Capability [C] . Yu Zhao, Sam Bearden, Guigen Zhang Society for Biomaterials annual meeting and exposition . 2019

机译：较少探索的表面性质：电双层及其分子询问能力
5. Molecular physics of electrical double layers in electrochemical capacitors. [D] . Feng, Guang. 2010

机译：电化学电容器中双电层的分子物理学。
6. A Polymer Blend Electrolyte Based on CS with Enhanced Ion Transport and Electrochemical Properties for Electrical Double Layer Capacitor Applications [O] . Shujahadeen B. Aziz, Elham M. A. Dannoun, Muhamad H. Hamsan, 2021

机译：基于CS的聚合物混合电解质具有增强的离子传输和用于电双层电容器应用的电化学性能
7. Molecular dynamics simulations of the electrical double layer on smectite surfaces contacting concentrated mixed electrolyte (NaCl-CaCl2) [O] . Bourg, I.C., Sposito, G. 2011

机译：接触浓缩混合电解质（NaCl-CaCl2）的蒙脱石表面双电层的分子动力学模拟
8. Molecular Dynamics Simulations of the Electrical Double Layer on Smectite Surfaces Contacting Concentrated Mixed Electrolyte (nCl-CaCl2) Solutions. [R] . Bourg, I. C., Sposito, G. 2011

机译：接触浓缩混合电解质（nCl-CaCl2）溶液的蒙脱石表面双电层的分子动力学模拟。

A Less-Explored Surface Property: The Electrical Double Layer and Its Molecular Interrogation Capability

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