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High-temperature DMMP combustion measurements in a shock tube using laser absorption spectroscopy

机译：使用激光吸收光谱法在冲击管中进行高温DMMP燃烧测量

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Pyrolysis of DMMP - a simulant for sarin-GB has been carried out at temperature range of 1300-1800K and around 1 atm pressure. Intermediate species concentrations (CO and CH_4) were measured using 4.6um laser and 3400 nm laser respectively. Laser diagnostics scheme for DMMP detection and measurement was developed at 9.569 um using C02 gas laser. Future work is to obtain time resolved data for decomposition of the parent compound using the new diagnostic. From the preliminary experiments, it was found that LLNL model underpredicts CO yield during DMMP pyrolysis. The experimental data collected in this study will be extremely useful in refinement and validation of kinetic model for combustion of OPC simulants.

机译：DMMP的热解-沙林-GB的模拟物已在1300-1800K的温度范围和约1个大气压的压力下进行。分别使用4.6um激光和3400 nm激光测量中间物种浓度（CO和CH_4）。使用CO2气体激光器在9.569 um处开发了用于DMMP检测和测量的激光诊断方案。未来的工作是使用新的诊断程序获取时间分解数据，以分解母体化合物。从初步实验中发现，LLNL模型在DMMP热解过程中低估了CO的收率。在这项研究中收集的实验数据将对OPC模拟物燃烧的动力学模型的完善和验证非常有用。

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《AIAA SciTech Forum and Exposition》|2020年|1003-1006|共4页
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Sneha Neupane; Samuel Barak; Erik Ninnemann; Ramees Rahman; Artem Masunov; Subith Vasu;
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1. DMMP pyrolysis and oxidation studies at high temperature inside a shock tube using laser absorption measurements of CO [J] . Neupane Sneha, Rahman Ramees K., Baker Jessica, Combustion and Flame . 2020,第Apra期

机译：使用CO的激光吸收测量，在冲击管内高温下的DMMP热解和氧化研究
2. Shock-Tube Laser Absorption Measurements of CO and H_2O during Iso-Octane Combustion [J] . Mathieu O., Cooper S. P., Alturaifi S., Energy & fuels . 2020,第6期

机译：异辛烷燃烧过程中CO和H_2O的冲击管激光吸收测量
3. Corrigendum to 'Assessment of modern detailed kinetics mechanisms to predict CO formation from methane combustion using shock-tube laser-absorption measurements' [Fuel 236 (2019) 1164-1180] [J] . Mathieu Olivier, Mulvihill Clayton R., Petersen Eric L. Fuel . 2019,第APRa15期

机译：“使用冲击管激光吸收测量法评估现代详细动力学机制以预测甲烷燃烧产生的二氧化碳形成”的勘误[燃料236（2019）1164-1180]
4. Sarin simulant combustion at high temperature: Time resolved laser absorption spectroscopy of intermediate products in a shock tube [C] . Sneha Neupane, Frank Barnes, Samuel Barak, AIAA aerospace sciences meeting;AIAA SciTech forum . 2018

机译：高温下的沙林模拟燃烧：冲击管中中间产物的时间分辨激光吸收光谱
5. Shock tube measurements of elementary oxidation and decomposition reactions important in combustion using hydroxide, methylidyne and nitrogen-carbon-nitrogen laser absorption. [D] . Vasudevan, Venkatesh. 2007

机译：使用氢氧化物，亚甲基炔烃和氮-碳-氮激光吸收对燃烧中重要的基本氧化和分解反应的冲击管测量。
6. Towards simultaneous measurements of electronic and structural properties in ultra-fast x-ray free electron laser absorption spectroscopy experiments [O] . J. Gaudin, C. Fourment, B. I. Cho, -1

机译：在超快速X射线自由电子激光吸收光谱实验中同时测量电子和结构性质
7. High-temperature iso-butene absorption diagnostic for shock tube kinetics using a pulsed quantum cascade laser near 11.3 μm [O] . R.M. Spearrin, S. Li, D.F. Davidson, 2015

机译：使用脉冲量子级联激光接近11.3μm的脉冲量子级联激光，高温异丁烯吸收诊断诊断
8. High Temperature Kinetic Study of the Reactions H + O2 = OH + O and O + H2 = OH +H in H2/O2 System by Shock Tube-Laser Absorption Spectroscopy [R] . Ryu, S., Hwang, S. M., Dewitt, K. J. 1995

机译：冲击管 - 激光吸收光谱法研究H2 / O2体系反应中H + O2 = OH + O和O + H2 = OH + H的高温动力学研究

High-temperature DMMP combustion measurements in a shock tube using laser absorption spectroscopy

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