DIELECTRIC RELAXATION SPECTROSCOPY FOR PROBING ION/NETWORK INTERACTIONS IN SOLIDS

机译：固体中离子/网络相互作用的介电弛豫谱

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It is emphasised that the comparison of Complex Impedance Spectroscopy (CIS) and of Thermally Stimulated Current (TSC) helps to gain a better understanding on the electrical response of ionic solids. More particularly, it allows us to isolate the "pure" dielectric contribution from the whole electrical signal. It is pointed out that the analysis of the dielectric behaviour can lead to obtain important information about the localisation of ions into a given structure and to determine the energy which characterises the interaction between ions and their surrounding network. Thus, for instance, the impact of the cationic exchange in zeolite or in oxide glasses can be quantified. Also, we show it can be a starting point for modelling ionic displacement mechanisms as well as, in a broader scope, the nature of ionic bonds in solids.

机译：需要强调的是，复阻抗谱（CIS）和热激励电流（TSC）的比较有助于更好地理解离子固体的电响应。更具体地说，它使我们能够将“纯”介电贡献与整个电信号隔离开来。要指出的是，对介电行为的分析可以导致获得有关离子在给定结构中的定位的重要信息，并可以确定表征离子与其周围网络之间相互作用的能量。因此，例如，可以定量阳离子交换在沸石或氧化物玻璃中的影响。同样，我们表明它可以作为模拟离子置换机理以及在更广泛的范围内固体中离子键性质的起点。

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来源
《NATO Advanced Study Institute on New Trends in Intercalation Compounds for Energy Storage, Sep 22-Oct 2, 2001, Sozopol, Bulgaria》|2001年|p.413-420|共8页
会议地点 Sozopol(BG)
作者
F. HENN; S. DEVAUTOUR; J.C. GIUNTINI;
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作者单位

Laboratoire de Physicochimie de la Matiere Condensee, CC003 UMR 5617 CNRS, Universite Montpellier II 34095 Montpellier, France;

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正文语种 eng
中图分类能源与动力工程;
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DIELECTRIC RELAXATION SPECTROSCOPY FOR PROBING ION/NETWORK INTERACTIONS IN SOLIDS

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