Double Pulse Laser deposition of polymer Nanocomposite: NaYF_4:Tm~(3+),Yb~(3+) films for optical sensors and light emitting applications

机译：聚合物纳米复合材料的双脉冲激光沉积：NaYF_4：Tm〜（3 +），Yb〜（3+）膜，用于光学传感器和发光应用

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The main objective of this paper is to demonstrate the feasibility of producing operationally Nanocomposite polymeric thin films for sensor and light emitting applications using the innovative modified double pulsed laser deposition (DPLD) technique. The existing PLD vacuum chamber was modified to accommodate multiple wavelength laser beams for in-situ-double-ablation/Deposition (DPLD) of multiple targets of host and dopants. Special design was made for cooling of the target to the threshold of the polymer ablation without interrupting the continuity of the ablation process. Multi-layered of nanocomposites of acrylic polymers and nanoparticles of NaYF_4:Tm~(3+),Yb~(3+)are fabricated using ultra-violet (UV) radiation (355 nm) ablating polymer targets and near-infra-red (near-IR) radiation (1064 nm) ablating inorganic targets. The films were characterized using the reflected high energy electron diffraction (RHEED), XRD , XRF, AFM, and FTIR absorption spectroscopy and tested as possible chemical sensors and light emitters.

机译：本文的主要目的是证明使用创新的改良双脉冲激光沉积（DPLD）技术生产用于传感器和发光应用的可操作纳米复合聚合物薄膜的可行性。对现有的PLD真空室进行了修改，以容纳多波长激光束，以便对主体和掺杂剂的多个目标进行原位双烧蚀/沉积（DPLD）。进行了特殊设计，以将靶材冷却至聚合物烧蚀的阈值，而不会中断烧蚀过程的连续性。利用紫外（UV）辐射（355 nm）烧蚀聚合物靶材和近红外光谱仪制备了丙烯酸聚合物纳米复合材料和NaYF_4：Tm〜（3 +），Yb〜（3+）纳米颗粒的多层结构近红外（1064 nm）辐射烧蚀无机目标。使用反射高能电子衍射（RHEED），XRD，XRF，AFM和FTIR吸收光谱对膜进行表征，并测试它们是否可能作为化学传感器和发光体。

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《Photonic fiber and crystal devices: advances in materials and innovations in device applications VII》|2013年|884702.1-884702.13|共13页
会议地点 San Diego CA(US)
作者
Abdalla M Darwish; Simeon Wilson; Sergey Sarkisov; Darayas Patel;
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作者单位

Physics Department, Dillard University, New Orleans , LA 70122;

Physics Department, Dillard University, New Orleans , LA 70122;

SSS optical Technologies, 515 Sparkman Drive, Suite 122 Huntsville, AL 35816-3417;

Oakwood University, Department of Mathematics Computer Science, 7000 Adventist Blvd., Huntsville, AL 35896;

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正文语种 eng
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Double Pulse Laser deposition; polymeric thin film; Nanocomposite; NaYF_4:Tm~(3+),Yb~(3+); optical sensors; light emitting applications; RHEED; XRD; XRF; FTIR;

机译：双脉冲激光沉积；聚合物薄膜纳米复合材料NaYF_4：Tm〜（3 +），Yb〜（3+）;光学传感器发光应用； RHEED； XRD; XRF;红外光谱;

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1. Preparation of NaYF_4: Gd~(3+), Yb~(3+), Tm~(3+) @ TiO_2 and NaYF_4: Gd~(3+), Yb~(3+), Tm~(3+) @ TiO_2 @ Au nanocomposites and their upconversion and photocatalytic properties under simulated solar light with or without an UV filter [J] . Shuwang Duo, Cuiping Zhong, JieJun Zhang, Journal of materials science . 2018,第4期

机译：NaYF_4的制备：Gd〜（3+），Yb〜（3+），Tm〜（3+）@ TiO_2和NaYF_4：Gd〜（3+），Yb〜（3+），Tm〜（3+）@带有或不带有紫外线滤光片的模拟太阳光下TiO_2 @ Au纳米复合材料及其上转换和光催化性能
2. Upconversion Luminescence Properties of Yb~(3+) and Tm~(3+) Codoped Amorphous Fluoride ZrF_4-BaF_2-LaF_3-AlF_3-NaF Thin Film Prepared by Pulsed Laser Deposition [J] . Chunfeng He, Guanshi Qin, Dan Zhao, Journal of nanoscience and nanotechnology . 2014,第5期

机译：脉冲激光沉积制备Yb〜（3+）和Tm〜（3+）共掺杂非晶氟化物ZrF_4-BaF_2-LaF_3-AlF_3-NaF薄膜的上转换发光性能
3. Graphene supported βNaYF_4:Yb~(3+),Tm~(3+) and N doped P25 nanocomposite as an advanced NIR and sunlight driven upconversion photocatalyst [J] . Wei Wang, Wenjuan Huang, Yaru Ni, Applied Surface Science . 2013,第OCTa1期

机译：石墨烯负载的βNaYF_4：Yb〜（3 +），Tm〜（3+）和N掺杂的P25纳米复合材料作为先进的近红外和阳光驱动的上转换光催化剂
4. Double Pulse Laser deposition of polymer Nanocomposite: NaYF_4:Tm~(3+),Yb~(3+) films for optical sensors and light emitting applications [C] . Abdalla M Darwish, Simeon Wilson, Sergey Sarkisov, Conference on photonic fiber and crystal devices: advances in materials and innovations in device applications VII . 2013

机译：双脉冲激光沉积聚合物纳米复合材料：NayF_4：Tm〜（3 +），Yb〜（3+）光学传感器和发光应用的薄膜
5. Power scaling of diode-pumped Nd(3+) and Yb(3+)-Doped YCa(4)O(BO(3))(3) (YCOB): A new self-frequency doubling laser. [D] . Hammons, Dennis Allen. 2000

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机译：NaGdF _{4 ：Nd ^{3 + ，Yb ^{3 + ，Tm ^{3 + 具有上转换的纳米晶体的磁和光学性质/下转换发光，从可见光到近红外第二窗口}}}}
8. Room temperature CW laser efficiency of Yb(sup 3+-)Er(sup 3+) and Tm(sup 3+) doped silicates in the infrared region [R] . Borel, C. , Souriau, J. C. , Wyon, C. , 1993

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Double Pulse Laser deposition of polymer Nanocomposite: NaYF_4:Tm~(3+),Yb~(3+) films for optical sensors and light emitting applications

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