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Strong non-linear MCD-effects due to partially circular polarized light sources

机译:部分圆偏振光源引起的强烈的非线性MCD效应

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Most soft x-ray magnetic dichroism studies are carried out with light of mixed polarization. The effect of incomplete circular polarization is usually taken care off by linearly extrapolating the data to P_circ=1. Using a classical model which includes the polarization factor we show that the MCD-effect, which is the normalized quantity 2(I~+ -I~-)/(I~+ +I~-), is highly non-linear with regard to P_circ. With a specially designed quadruple reflection phase shifter we measrued the MCD effect with P_circ<1 as well as with P_circ approx 1. MCD spectra of Fe around the M_2,3 transition verify our model calculationsof the polarization dependence. The data indicate that the observed non-linear response of the MCD-effect to P-circ can generally introduce large errorsin the quantitative analysis of MCD data where spin and orbital moments are extracted by means of sum rules.
机译:大多数软X射线磁二向色性研究都是使用混合偏振光进行的。通常通过将数据线性外推到P_circ = 1来消除不完全圆极化的影响。使用包含极化因子的经典模型,我们表明MCD效应(归一化量2(I〜+ -I〜-)/(I〜+ + I〜-))在高度非线性方面至P_circ。使用专门设计的四重反射移相器,我们测量了P_circ <1以及P_circ约为1的MCD效应。M_2,3跃迁附近的Fe的MCD光谱验证了我们对偏振相关性的模型计算。数据表明,观察到的MCD效应对P圆的非线性响应通常会在MCD数据的定量分析中引入较大的误差,其中通过求和规则提取自旋和轨道矩。

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