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Nanoscale thermal, acoustic, and magnetic dynamics probed with soft x-ray light.

机译:用软X射线探测纳米级的热,声和磁动力学。

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摘要

This thesis discusses the application of coherent, ultrafast beams of soft x-ray light from high-order harmonic generation (HHG) to study thermal, acoustic, and magnetic processes in nanostructures. This short-wavelength light is a uniquely powerful probe of surface dynamics since it has both a very short wavelength and duration.;First, this thesis reports the first observation and quantitative measurements of the transition from diffusive to ballistic thermal transport for the case of heat flow away from a heated nanostructure into a bulk substrate. This measurement provides insight into the fundamentals of thermal energy transport away from nanoscale hot spots, and demonstrates a fundamental limit to the energy dissipation capability of nanostructures. Further, we propose a straightforward correction to the Fourier law for heat diffusion, necessary for thermal management in nanoelectronics, nano-enabled energy systems, nanomanufacturing, and nanomedicine.;Second, this work discusses dynamic measurements of ultra-high frequency surface acoustic waves (SAW) and the first SAW dispersion measurement in a nanostructured system. These results are directly applicable to adhesion and thickness diagnostics of very thin films.;Finally, this thesis reports the first use of light from HHG to study magnetic orientation. Using the transverse magneto-optic Kerr effect and soft x-ray light near the M-absorption edges of Fe, Co, and Ni, magnetic asymmetries up to 8% are observed from thin Permalloy (Ni80Fe20) films. This signal is 1-2 orders of magnitude higher than that observed using optical methods, showing great promise for dynamic imaging of domain flipping at the 100 nm level.
机译:本文讨论了来自高次谐波产生(HHG)的软性X射线相干超快光束在研究纳米结构中的热,声和磁过程中的应用。这种短波长光具有非常短的波长和持续时间,是表面动力学的独特强大的探测器。首先,本论文报道了对热情况下从扩散热传递到弹道热传递的转换的首次观察和定量测量。从加热的纳米结构流到块状基材中。该测量提供了对热能从纳米级热点转移的基本原理的了解,并证明了对纳米结构的能量消散能力的根本限制。此外,我们建议对热扩散的傅立叶定律进行直接校正,这对于纳米电子学,纳米能量系统,纳米制造和纳米医学中的热管理是必不可少的;其次,本工作讨论了超高频表面声波的动态测量( SAW)和纳米结构系统中的首次SAW色散测量。这些结果直接适用于非常薄的薄膜的附着力和厚度诊断。最后,本文报道了HHG光首次用于研究磁取向。使用横向磁光Kerr效应和Fe,Co和Ni的M吸收边缘附近的软X射线光,从坡莫合金(Ni80Fe20)薄膜中观察到高达8%的磁不对称性。该信号比使用光学方法观察到的信号高1-2个数量级,这显示了在100 nm级别对域翻转进行动态成像的广阔前景。

著录项

  • 作者

    Siemens, Mark E.;

  • 作者单位

    University of Colorado at Boulder.;

  • 授予单位 University of Colorado at Boulder.;
  • 学科 Physics General.;Physics Condensed Matter.;Physics Optics.
  • 学位 Ph.D.
  • 年度 2009
  • 页码 195 p.
  • 总页数 195
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 物理学;光学;
  • 关键词

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