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Electronic structure and collective mode coupling in the single-layer high-temperature superconductor, Bi2201.

机译:单层高温超导体Bi2201中的电子结构和集体模式耦合。

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摘要

Perovskite metal-oxides are known to exhibit rich physical properties, including high-temperature superconductivity, Mott- and band-insulating states, colossal magnetoresistance, multiferroic states and polaron physics. For this interest, angle-resolved photoemission studies (ARPES) have been successfully preformed in elucidating the electronic properties of doped Mott insulators, especially high-temperature cuprate superconductors. In this thesis, I will present ARPES study of single-layer Bi2Sr2CuO 6 superconductor.;The first part focuses on the dispersion anomaly ("kink") of single-layer Bi2Sr2CuO6 superconductor. The motivation comes from that the coupling of electrons to bosonic modes is known to be the heart of mechanism of Cooper pair formation in conventional superconductors. For cuprate superconductors, evidence of electron-boson coupling has manifested itself in the form of the dispersion anomaly. The self-energies obtained from the kink are compared between optimally doped and strongly overdoped, non-superconducting samples. Besides the appearance of a strong overall weakening, it is also found that the weight of self-energy in the overdoped system shifts to higher energies. Evidence shows that this could be related to a change in the coupling to c-axis phonons due to the rapid change of the c-axis screening in this doping range.;In the second part, at higher-energy scale, we present improved experimental data from four families of high-Tc superconductors, including Bi2Sr2CuO6, over a wide doping range that reveal a hierarchy of many-body interaction scales focused on: the low-energy anomaly (above) of 0.03--0.09 eV, a high-energy anomaly of 0.3--0.5 eV, and an anomalous enhancement of the width of the local-density-approximation-based CuO2 band extending to energies of ≈2 eV. Besides their universal behavior over the families, we find that all of these three dispersion anomalies also show clear doping dependence over the doping range presented. Further study shows that the essential features of high-energy-anomaly can be captured rather well by the calculation based on the single-band Hubbard model.
机译:已知钙钛矿金属氧化物具有丰富的物理特性,包括高温超导性,莫特和带绝缘态,巨大的磁阻,多铁性态和极化子物理学。出于这种兴趣,已成功进行了角度分辨光发射研究(ARPES),以阐明掺杂的Mott绝缘子,尤其是高温铜酸盐超导体的电子性能。在本文中,我将介绍单层Bi2Sr2CuO6超导体的ARPES研究。第一部分着重于单层Bi2Sr2CuO6超导体的色散异常(“扭曲”)。动机来自于将电子耦合至波速模式是常规超导体中库珀对形成机理的核心。对于铜酸盐超导体,电子-玻色子耦合的证据以色散异常的形式表现出来。比较从扭结获得的自能量在最佳掺杂和强过量掺杂的非超导样品之间。除了出现整体强弱减弱的现象外,还发现过量掺杂的系统中自能量的权重转移到了更高的能量上。有证据表明,这可能是由于在此掺杂范围内c轴筛选的快速变化导致与c轴声子耦合的变化所致。第二部分,在较高能级下,我们提出了改进的实验来自四个高Tc超导体家族的数据,包括Bi2Sr2CuO6,在宽的掺杂范围内揭示了多体相互作用尺度的层次结构,该尺度着重于:0.03--0.09 eV的低能异常(上),高能0.3--0.5 eV的异常值,并且基于局部密度近似的CuO2谱带的宽度异常增大,扩展到≈ 2 eV的能量。除了它们在族上的普遍行为外,我们发现所有这三个色散异常在所显示的掺杂范围内也显示出明显的掺杂依赖性。进一步的研究表明,通过基于单频带Hubbard模型的计算,可以很好地捕获高能异常的基本特征。

著录项

  • 作者

    Meevasana, Worawat.;

  • 作者单位

    Stanford University.;

  • 授予单位 Stanford University.;
  • 学科 Physics Condensed Matter.
  • 学位 Ph.D.
  • 年度 2009
  • 页码 160 p.
  • 总页数 160
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 O49;
  • 关键词

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