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Electron transport in single molecule magnet transistors and optical transitions in the 15nitrogen-vacancy- center in diamond.

机译:单分子磁性晶体管中的电子传输和金刚石中15氮空位中心的光学跃迁。

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摘要

This thesis presents theoretical studies dealing with quantum interference effects in electron transport through single molecule magnet transistors and a study on optical Λ transitions in the 15NV - center in diamond. The thesis starts with a brief general introduction to the physics of quantum transport through single electron transistors. Afterwards, the main body of the thesis is divided into three studies: (i) In chapter (2) we describe the properties of single molecule magnets and the Berry phase interference present in these nanomagnets. We then propose a way to detect quantum interference experimentally in the current of a single molecule magnet transistor using polarized leads. We apply our theoretical results to the newly synthesized nanomagnet Ni4. (ii) In chapter (3) we review the Kondo effect and present a microscopic derivation of the Kondo Hamiltonian suitable for full and half-integer spin nanomagnets. We then calculate the conductance of the single molecule magnet transistor in the presence of the Kondo effect for Ni4 and show how the Berry phase interference becomes temperature dependent. (iii) We conclude in chapter (4) with a theoretical study of the single Nitrogen vacancy defect center in diamond. We show that it is possible to have spin non-conserving transitions via the hyperfine interaction and propose a way to write and read quantum information using circularly polarized light by means of optical Λ transitions in this solid state system.
机译:本文提出了有关通过单分子磁性晶体管的电子传输中的量子干扰效应的理论研究,以及对金刚石15NV中心的光学Λ跃迁的研究。本文首先简要介绍了通过单电子晶体管进行量子传输的物理学。此后,论文的主体分为三个研究:(i)在第(2)章中,我们描述了单分子磁体的特性以及这些纳米磁体中存在的Berry相干涉。然后,我们提出了一种使用极化引线在实验中检测单分子磁性晶体管电流中的量子干扰的方法。我们将理论结果应用于新合成的纳米磁体Ni4。 (ii)在第(3)章中,我们回顾了近藤效应,并提出了适用于全整数和半整数自旋纳米磁体的近藤哈密顿量的微观推导。然后,我们在存在Ni4的Kondo效应的情况下计算单分子磁性晶体管的电导,并显示Berry相干扰如何与温度有关。 (iii)我们在第(4)章结束时对金刚石中单个氮空位缺陷中心进行了理论研究。我们表明,通过超精细相互作用可能具有自旋非保守跃迁,并提出了一种在该固态系统中利用光学Λ跃迁使用圆偏振光写入和读取量子信息的方法。

著录项

  • 作者

    Gonzalez, Gabriel.;

  • 作者单位

    University of Central Florida.;

  • 授予单位 University of Central Florida.;
  • 学科 Physics Condensed Matter.
  • 学位 Ph.D.
  • 年度 2009
  • 页码 128 p.
  • 总页数 128
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

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