首页> 中文期刊> 《安徽地质》 >Computational Study of Ternary Devices:Stable, Low-Cost, and Efficient Planar Perovskite Solar Cells

Computational Study of Ternary Devices:Stable, Low-Cost, and Efficient Planar Perovskite Solar Cells

         

摘要

Although perovskite solar cells with power con-version efficiencies (PCEs) more than 22%have been realized with expensive organic charge-transporting materials, their stability and high cost remain to be addressed. In this work, the perovskite configuration of MAPbX (MA=CH3NH3, X=I3, Br3, or I2Br) integrated with stable and low-cost Cu:NiOx hole-transporting material, ZnO electron-transport-ing material, and Al counter electrode was modeled as a planar PSC and studied theoretically. A solar cell simulation program (wxAMPS), which served as an update of the popular solar cell simulation tool (AMPS:Analysis of Microelectronic and Photonic Structures), was used. The study yielded a detailed understanding of the role of each component in the solar cell and its effect on the photovoltaic parameters as a whole. The bandgap of active materials and operating temperature of the modeled solar cell were shown to influence the solar cell performance in a significant way. Further, the simulation results reveal a strong dependence of photovoltaic parameters on the thickness and defect density of the light-absorbing layers. Under moderate simulation conditions, the MAPbBr3 and MAPbI2Br cells recorded the highest PCEs of 20.58 and 19.08%, respectively, while MAPbI3 cell gave a value of 16.14%.

著录项

  • 来源
    《安徽地质》 |2018年第3期|142-152|共11页
  • 作者单位

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    Electronic and Magnetic Materials Department, Advanced Materials Division, Central Metallurgical Research and Development Institute (CMRDI), P.O. Box 87, Helwan, Cairo 11421, Egypt;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

    State Key Laboratory of Alternate Electrical Power, System with Renewable Energy Sources, School of Renewable Energy, North China Electric Power University, Beijing 102206, People's Republic of China;

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