Designing of highly selective and high-temperature endurable RWGS heterogeneous catalysts: recent advances and the future directions

Xiong Su; Xiaoli Yang; Bo Zhao; Yanqiang Huang

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Designing of highly selective and high-temperature endurable RWGS heterogeneous catalysts: recent advances and the future directions

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Reverse water gas shift (RWGS) reaction can be served as a pivotal stage of transitioning the abundant CO2 resource into chemicals or hydrocarbon fuels,which is attractive for the CO2 utilization and of eventually significance in enabling a rebuilt ecological system for unconventional fuels.This concept is appealing when the process is considered as a solution for the storage of renewable energy,which may also find a variety of potential end uses for the outer space exploration.However,a big challenge to this issue is the rational design of high temperature endurable RWGS catalysts with desirable CO product selectivity.In this work,we present a comprehensive overview of recent publications on this research topic,mainly focusing on the catalytic performance of RWGS reaction over three major kinds of heterogeneous catalysts,including supported metal catalysts,mixed oxide catalysts and transition metal carbides.The reaction thermodynamic analysis,kinetics and mechanisms are also described in detail.The present review attempts to provide a general guideline about the construction of well-performed heterogeneous catalysts for the RWGS reaction,as well as discussing the challenges and further prospects of this process.

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《天然气化学（英文版）》 |2017年第5期|854-867|共14页
作者
Xiong Su; Xiaoli Yang; Bo Zhao; Yanqiang Huang;
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iChEM(Collaborative Innovation Center of Chemistry for Energy Materials), Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;

iChEM(Collaborative Innovation Center of Chemistry for Energy Materials), Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;

University of Chinese Academy of Sciences, Beijing 100049, China;

Renewable Energy Storage Division, Global Energy Interconnection Research Institute(GEIRI), Future Science and Technology City, Beijing 102211, China;

iChEM(Collaborative Innovation Center of Chemistry for Energy Materials), Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;

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Designing of highly selective and high-temperature endurable RWGS heterogeneous catalysts: recent advances and the future directions

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