Hydrogen generation with acid/alkaline amphoteric water electrolysis

Qing Lei; Baoguo Wang; Peican Wang; Shuai Liu

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Hydrogen generation with acid/alkaline amphoteric water electrolysis

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To reduce the energy consumption of the electrolytic hydrogen generation process, we propose a novel approach to generate hydrogen with acidic/alkaline amphoteric water electrolysis, wherein hydrogen is produced inside an acidic solution and oxygen evolved under alkaline condition, and a membrane is employed in the middle of the electrolyzer to restrain neutralization. The electrode polarization is greatly reduced due to the specific arrangement of the acidic/alkaline amphoteric electrolyzer. The rate of hydrogen production achieves over four times higher than that of the alkaline aqueous solution at 2.2 V, and the energy consumption is reduced approximately 30% under the current density of 200 m A/cm ^2. The investigation of transmembrane potential drop indicates water splitting on the membrane surfaces, which compensates for acid or alkaline loss on-site and maintains the concentration approximately constant during electrolysis process. The acidic/alkaline amphoteric water electrolysis is promising as an energy saving, clean and sustainable hydrogen production technology.

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《天然气化学（英文版）》 |2019年第11期|162-169|共8页
作者
Qing Lei; Baoguo Wang; Peican Wang; Shuai Liu;
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The State Key Laboratory of Chemical Engineering Department of Chemical Engineering Tsinghua University Beijing 100084 China;

The State Key Laboratory of Chemical Engineering Department of Chemical Engineering Tsinghua University Beijing 100084 China;

The State Key Laboratory of Chemical Engineering Department of Chemical Engineering Tsinghua University Beijing 100084 China;

The State Key Laboratory of Chemical Engineering Department of Chemical Engineering Tsinghua University Beijing 100084 China;

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Hydrogen generation with acid/alkaline amphoteric water electrolysis

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