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Elucidating the Mechanisms of Two Unique Phenomena Governed by Particle-Particle Interaction under DEP: Tumbling Motion of Pearl Chains and Alignment of Ellipsoidal Particles

机译:阐明在DEP下由粒子与粒子相互作用控制的两个独特现象的机理:珍珠链的翻滚运动和椭球的排列

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摘要

Particle-particle interaction plays a crucial role in determining the movement and alignment of particles under dielectrophoresis (DEP). Previous research efforts focus on studying the mechanism governing the alignment of spherical particles with similar sizes in a static condition. Different approaches have been developed to simulate the alignment process of a given number of particles from several up to thousands depending on the applicability of the approaches. However, restricted by the simplification of electric field distribution and use of identical spherical particles, not much new understanding has been gained apart from the most common phenomenon of pearl chain formation. To enhance the understanding of particle-particle interaction, the movement of pearl chains under DEP in a flow condition was studied and a new type of tumbling motion with unknown mechanism was observed. For interactions among non-spherical particles, some preceding works have been done to simulate the alignment of ellipsoidal particles. Yet the modeling results do not match experimental observations. In this paper, the authors applied the newly developed volumetric polarization and integration (VPI) method to elucidate the underlying mechanism for the newly observed movement of pearl chains under DEP in a flow condition and explain the alignment patterns of ellipsoidal particles. The modeling results show satisfactory agreement with experimental observations, which proves the strength of the VPI method in explaining complicated DEP phenomena.
机译:颗粒间相互作用在决定介电电泳(DEP)下颗粒的运动和排列中起着至关重要的作用。先前的研究工作集中于研究在静态条件下控制尺寸相似的球形颗粒排列的机理。已经开发了不同的方法来模拟给定数量的粒子的排列过程,该方法取决于方法的适用性,从几到数千。然而,受电场分布简化和使用相同球形颗粒的限制,除了最常见的珍珠链形成现象外,没有获得太多新的认识。为了增进对粒子间相互作用的理解,研究了流动条件下DEP下珍珠链的运动,并观察到一种新型的翻滚运动,其机理尚不清楚。对于非球形粒子之间的相互作用,已经进行了一些先前的工作来模拟椭圆形粒子的排列。然而,建模结果与实验观察结果不符。在本文中,作者应用了最新开发的体积极化和积分(VPI)方法,阐明了在流动条件下在DEP条件下新观察到的珍珠链运动的潜在机理,并解释了椭圆形颗粒的排列方式。建模结果与实验观察结果令人满意,证明了VPI方法在解释复杂的DEP现象方面的优势。

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