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Photochromic benzobphosphole oxide with excellent thermal irreversibility and fatigue resistance in the thin film solid state via direct attachment of dithienyl units to the weakly aromatic heterocycle

机译：通过将二噻吩基单元直接连接到弱芳族杂环上而在薄膜固态下具有出色的热不可逆性和抗疲劳性的光致变色苯并b磷氧化物

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摘要

A novel photochromic benzo[b]phosphole oxide has been demonstrated to display photochromic properties with excellent fatigue resistance and thermal irreversibility in polymethylmethacrylate (PMMA) thin film under ambient conditions. The remarkable photochromic behaviour can be achieved by rational molecular design, in which the weakly aromatic phosphole oxide is directly incorporated into the photo-responsive dithienylethene units. Photopatterning via photoinduced colouration and decolouration has been performed to demonstrate the repeatable and distinct transformation between the bistable states, making it a promising candidate with photoswitching properties for optoelectronic applications.

机译：新型光致变色苯并[b]磷氧化物已证明在环境条件下在聚甲基丙烯酸甲酯（PMMA）薄膜中具有优异的抗疲劳性和热不可逆性，具有光致变色性能。通过合理的分子设计可以实现显着的光致变色行为，其中将弱芳族的氧化磷直接掺入光响应性二噻吩基乙烯单元中。已经进行了通过光致着色和脱色的光图案化，以证明双稳态之间可重复且独特的转变，使其成为具有光开关特性的光电子应用的有希望的候选者。

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期刊名称 Chemical Science
作者
Nathan Man-Wai Wu; Hok-Lai Wong; Vivian Wing-Wah Yam;
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作者单位

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年(卷),期 2017(8),2
年度 2017
页码 1309–1315
总页数 7
原文格式 PDF
正文语种
中图分类生化遗传学;生化药理学;
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1. Photochromic benzo[b]phosphole oxide with excellent thermal irreversibility and fatigue resistance in the thin film solid state via direct attachment of dithienyl units to the weakly aromatic heterocycle [J] . Nathan Man-Wai Wu, Hok-Lai Wong, Vivian Wing-Wah Yam Chemical science . 2017,第2期

机译：光致变色苯并[ b ]氧化磷在薄膜固态中具有出色的热不可逆性和抗疲劳性，通过二噻吩基单元直接连接到弱芳族杂环上

2. Photochromic benzo[b]phosphole oxide with excellent thermal irreversibility and fatigue resistance in the thin film solid state via direct attachment of dithienyl units to the weakly aromatic heterocycle [J] . Nathan Man-Wai Wu, Hok-Lai Wong, Vivian Wing-Wah Yam Chemical science . 2016,第2期

机译：光致变色苯并[B]磷酸氧化物，具有优异的热不可逆性和薄膜固态的疲劳性，通过直接附着二烯基单元到弱芳族杂环

3. Thermal conductivity and thermal boundary resistance of atomic layer deposited high-k dielectric aluminum oxide, hafnium oxide, and titanium oxide thin films on silicon [J] . Ethan A. Scott, John T. Gaskins, Sean W. King, APL Materials . 2018,第5期

机译：原子层在硅上沉积的高k电介质氧化铝，氧化ha和氧化钛薄膜的热导率和热边界电阻

4. Fabrication and Resistance-Switching Behaviors of NiO Thin films by Thermal Oxidation of Evaporated Ni Films [C] . X. Cao, X. M. Li, W. D. Yu, International Symposium on Advanced Synthesis and Processing Technology for Materials . 2009

机译：通过蒸发Ni膜的热氧化通过氧化NiO薄膜的制造和电阻切换行为

5. Direct synthesis and characterization of optically transparent conformal zinc oxide nanocrystalline thin films by rapid thermal plasma CVD [O] . Joachim D Pedersen, Heather J Esposito, Kwok Siong Teh 2011

机译：快速热等离子体CVD直接合成并表征光学透明的保形氧化锌纳米晶薄膜

6. Photochromic benzo[b]phosphole oxide with excellent thermal irreversibility and fatigue resistance in the thin film solid state via direct attachment of dithienyl units to the weakly aromatic heterocycle [O] . Yam, VWW, Wong, HL, WU, MW 2016

机译：光致变色苯并[b]磷杂环氧化物，通过直接连接二噻吩基单元到弱芳香杂环，在薄膜固态下具有优异的热不可逆性和抗疲劳性

7. Effect of grain orientation and coating on thermal fatigue resistance of a directionally solidified superalloy (MAR-M 247) [R] . Bizon, P. T., Dreshfield, R. L., Calfo, F. D. 1979

机译：晶粒取向和涂层对定向凝固高温合金（maR-m 247）抗热疲劳性能的影响

1. 空气诱导2-炔基苯基氧化磷环化合成苯并磷杂环戊二烯氧化物 [A] . 王文彪 . 2017

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3. FERRITIC STAINLESS STEEL EXCELLENT IN THERMAL FATIGUE PROPERTY, HIGH TEMPERATURE FATIGUE PROPERTY, OXIDATION RESISTANCE AND HIGH TEMPERATURE SALT DAMAGE CORROSION RESISTANCE [P] . 外国专利： JP2010053421A . 2010-03-11

机译：铁素体不锈钢在热疲劳性能，高温疲劳性能，抗氧化性和高温耐盐腐蚀性方面表现优异

4. FERRITIC STAINLESS STEEL EXCELLENT IN THERMAL FATIGUE PROPERTY, HIGH TEMPERATURE FATIGUE PROPERTY, OXIDATION RESISTANCE AND TOUGHNESS [P] . 外国专利： JP2010053420A . 2010-03-11

机译：铁素体不锈钢在热疲劳性能，高温疲劳性能，抗氧化性和韧性方面表现优异

5. FERRITIC STAINLESS STEEL EXCELLENT IN THERMAL FATIGUE PROPERTY, HIGH TEMPERATURE FATIGUE PROPERTY, OXIDATION RESISTANCE AND WORKABILITY [P] . 外国专利： JP2010053418A . 2010-03-11

机译：铁素体不锈钢在热疲劳性能，高温疲劳性能，抗氧化性和可加工性方面表现优异

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Photochromic benzobphosphole oxide with excellent thermal irreversibility and fatigue resistance in the thin film solid state via direct attachment of dithienyl units to the weakly aromatic heterocycle

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