首页> 美国卫生研究院文献>Scientific Reports >Possible Tomonaga-Luttinger spin liquid state in the spin-1/2 inequilateral diamond-chain compound K3Cu3AlO2(SO4)4
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Possible Tomonaga-Luttinger spin liquid state in the spin-1/2 inequilateral diamond-chain compound K3Cu3AlO2(SO4)4

机译:自旋1/2不等边菱形链化合物K3Cu3AlO2(SO4)4的可能Tomonaga-Luttinger自旋液体状态

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摘要

K3Cu3AlO2(SO4)4 is a highly one-dimensional spin-1/2 inequilateral diamond-chain antiferromagnet. Spinon continuum and spin-singlet dimer excitations are observed in the inelastic neutron scattering spectra, which is in excellent agreement with a theoretical prediction: a dimer-monomer composite structure, where the dimer is caused by strong antiferromagnetic (AFM) coupling and the monomer forms an almost isolated quantum AFM chain controlling low-energy excitations. Moreover, muon spin rotation/relaxation spectroscopy shows no long-range ordering down to 90 mK, which is roughly three orders of magnitude lower than the exchange interaction of the quantum AFM chain. K3Cu3AlO2(SO4)4 is, thus, regarded as a compound that exhibits a Tomonaga-Luttinger spin liquid behavior at low temperatures close to the ground state.
机译:K3Cu3AlO2(SO4)4是高度一维自旋1/2不等边菱形链反铁磁体。在非弹性中子散射光谱中观察到了旋子连续体和自旋单二聚体激发,这与理论预测非常吻合:二聚体-单体复合结构,其中二聚体由强反铁磁(AFM)耦合引起并且单体形式几乎孤立的量子AFM链控制着低能量的激发。此外,μ自旋旋转/弛豫光谱显示没有低至90 mK的远距离有序,这比量子AFM链的交换相互作用低大约三个数量级。因此,K 3 Cu 3 AlO 2(SO 4)4被认为是在接近基态的低温下具有Tomonaga-Luttinger自旋液体行为的化合物。

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