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Propagation of terahertz waves in a monoclinic crystal BaGa4Se7

机译:太赫兹波在单斜晶体BaGa4Se7中的传播

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摘要

The complex symmetric dielectric tensor of a monoclinic crystal cannot be diagonalized by a space rotation operation in general, which poses a serious difficulty in analyzing the propagation of electromagnetic fields in monoclinic crystals so far. This propagation issue is discussed in a general case without using the index ellipsoid scheme. It is found that, when incident waves travel along the mirror plane normal or 2-fold rotation axis of monoclinic crystals, two eigenmodes following specific dispersion relations are elliptically polarized with the same ellipticity and chirality but have spatially orthogonal elliptical principal axes. The frequency independent features are the unique manifestation of the crystal symmetry. Using polarization sensitive terahertz time-domain spectroscopy and our developed data analyzing and processing methods, three complex permittivity tensor elements for a monoclinic crystal BaGa4Se7 are straightforwardly extracted and the properties of the two eigenmodes are characterized in full. It is also interesting that the spectral components beyond 1.7 THz show a very high refraction index (>10) and low dissipation during propagation, which suggests that the bulk phonon-polariton waves may be excited and effectively propagate in the crystal, resulting from the coherent phonon excitations by the incident terahertz waves. Our results may promote to develop novel terahertz devices based on polariton excitation and propagation in monoclinic crystals.
机译:通常,单斜晶晶体的复对称介电张量不能通过空间旋转操作来对角线化,这迄今在分析电磁场在单斜晶晶体中的传播方面具有严重的困难。通常不使用索引椭球方案讨论此传播问题。发现,当入射波沿着单斜晶体的镜面法线或2倍旋转轴传播时,遵循特定色散关系的两个本征模以相同的椭圆率和手性被椭圆偏振,但是具有空间正交的椭圆主轴。频率无关的特征是晶体对称性的独特表现。利用偏振敏感太赫兹时域光谱技术和我们开发的数据分析和处理方法,直接提取了单斜晶体BaGa4Se7的三个复介电常数张量元素,并充分表征了两个本征模的性质。有趣的是,超过1.7 THz的光谱分量在传播过程中表现出很高的折射率(> 10)和低耗散,这表明由于相干效应,体声子-极化子波可能被激发并有效地在晶体中传播。入射的太赫兹波激发声子。我们的结果可能会促进开发基于极化子激发和单斜晶体中传播的新型太赫兹器件。

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