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Coherent anti-Stokes Raman spectroscopy utilizing phase mismatched cascaded quadratic optical interactions in nonlinear crystals

机译：利用非线性晶体中相位失配的级联二次光学相互作用的相干反斯托克斯拉曼光谱

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摘要

We experimentally investigated the nonlinear optical interaction between the instantaneous four-wave mixing and the cascaded quadratic frequency conversion in commonly used nonlinear optical KTP and LiNbO3 with the aim of a possible background suppression of the non-resonant background in coherent anti-Stokes Raman scattering. The possibility of background-free heterodyne coherent anti-Stokes Raman scattering microspectroscopy is investigated at the interface formed by a liquid (isopropyl alcohol) and a nonlinear crystal (LiNbO3).

机译：我们实验研究了常用的非线性光学KTP和LiNbO3中瞬时四波混频和级联二次频率转换之间的非线性光学相互作用，目的是可能抑制相干反斯托克斯拉曼散射中的非共振本底。在由液体（异丙醇）和非线性晶体（LiNbO3）形成的界面上研究了无背景外差相干反斯托克斯拉曼散射显微光谱的可能性。

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期刊名称 Optics Express
作者
Georgi I. Petrov; Miaochan Zhi; Vladislav V. Yakovlev;
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作者单位

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年(卷),期 -1(21),26
年度 -1
页码 31960–31965
总页数 6
原文格式 PDF
正文语种
中图分类情报学;
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1. Manifestations of nonlinear optical effects in a novel SRS-active crystal - natural topaz, Al_2(F_(1-x)(OH)_x)_2SiO_4: many-phonon Χ~(3)-lasing, more than sesqui-octave Stokes and anti-Stokes multi-wavelength comb lasing, cascaded and cross-cascaded Χ~(3) <-> Χ~(3) Raman-induced interactions under single-and dual-wavelength picosecond collinear coherent pumping, THG and combined SRS-promoting phonon modes [J] . A. A. Kaminskii, O. Lux, H. Rhee, Laser physics letters . 2013,第7期

机译：新型SRS活性晶体-天然黄玉Al_2（F_（1-x）（OH）_x）_2SiO_4的非线性光学效应的表现：多声子Χ〜（3）激光，比倍半倍频程斯托克斯和反-斯托克斯多波长梳状激射，级联和交叉级联的X〜（3）<-> X〜（3）在单波长和双波长皮秒共线相干泵浦，THG和SRS促进声子组合模式下的拉曼诱导相互作用
2. Nonresonant background suppression in coherent anti-Stokes Raman spectroscopy through cascaded nonlinear optical interactions [J] . Georgi I. Petrov, Miaochan Zhi, Dawei Wang, Optics Letters . 2013,第9期

机译：级联的非线性光学相互作用在相干反斯托克斯拉曼光谱中的非共振本底抑制
3. Stimulated Raman scattering in natural crystals of SrSO_4, BaSO_4 and PDSO_4: High-order Stokes and anti-Stokes generation with single-wavelength UV, visible, and near-IR excitation, as well as cascaded up-conversion nonlinear x~((3)) ↔ x ~((3)) lasing effects under dual-wavelength picosecond collinear coherent pumping [J] . A.A. Kaminskii, L. Bohaty, P. Becker, Applied physics . 2011,第2期

机译：SrSO_4，BaSO_4和PDSO_4天然晶体中的受激拉曼散射：具有单波长UV，可见光和近红外激发以及级联上转换非线性x〜（（3））的高阶斯托克斯和反斯托克斯生成）x〜（（3））在双波长皮秒共线相干泵浦下的激射效应
4. Generation of Ultrashort Optical Pulses Using Multiple Coherent Anti-Stokes Raman Scattering Signals in a Crystal and Observation of the Raman Phase [C] . International conference on ultrafast phenomena . 2009

机译：在晶体中使用多个相干抗箭头拉曼散射信号产生超短光脉冲的产生和拉曼阶段的观察
5. Waveguide Surface Coherent anti-Stokes Raman Scattering Spectroscopy and optical second harmonic generation spectroscopy of molecules adsorbed on metal oxide surfaces. [D] . Wijekoon, Wijekoon Mudiyanselage Kapila Piyasena. 1988

机译：波导表面相干抗斯托克斯拉曼散射光谱和光学二次谐波光谱，用于吸附在金属氧化物表面的分子。
6. Ex-CARS: exotic configuration for coherent anti-Stokes Raman scattering microspectroscopy utilizing two laser sources [O] . Vladislav V. Yakovlev, Georgi I. Petrov, Gary D. Noojin, -1

机译：EX-CARS：用于连贯的防斯托克斯拉曼散射微型光谱用两个激光源的异国配置
7. Ultrafast and octave-spanning optical nonlinearities from strongly phase-mismatched cascaded interactions [O] . Zhou, B. B., Chong, A., Wise, F. W., 2012

机译：超强和倍频程的光学非线性强烈相位不匹配的级联相互作用

Coherent anti-Stokes Raman spectroscopy utilizing phase mismatched cascaded quadratic optical interactions in nonlinear crystals

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