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Reticular Materials for Artificial Photoreduction of CO_2

机译：用于人工拍摄CO_2的网状材料

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Because of the energy crisis facing the planet, reducing fossil fuel reliance is an urgent scientific task. Alternative fuels have recently been in high demand. Taking into account the enormous amount of CO(2)released from combustion, converting CO(2)into high value-added products using photochemistry-the catalytic transformation is activated by the ubiquitous sunlight mimicking the photosynthesis of natural plants-is of paramount importance. Scientists have developed various photocatalysts for the CO(2)photoreduction. Among them, reticular materials including metal-organic frameworks (MOFs) and covalent organic frameworks (COFs) have been employed for many applications during the past decade and have emerged as advanced catalytic platforms for the photoreduction of CO2. This Progress Report aims to provide the fundamentals, mechanism, and methods of characterization to gain insight into the process of CO(2)photoreduction. In addition, this Progress Report highlights the achievements in using reticular materials as advanced catalysts for the photoreduction of CO(2)and discusses the relationship between structural features of MOFs/COFs with their photocatalytic performance. Based on the comprehension of advancements, opportunities, and challenges of reticular materials for the CO(2)photoreduction, the future prospects of this technology are discussed to direct the exciting research in designing better CO(2)reduction photocatalysts.
机译：由于面向地球的能量危机，减少化石燃料依赖是一种紧急的科学任务。最近需求的替代燃料已经很高。考虑到从燃烧中释放的巨大数量的CO（2），使用光化学将CO（2）转化为高附加值的产品 - 催化转化通过模拟天然植物的光合作用而激活 - 最重要的阳光是至关重要的。科学家们开发了各种光催化剂为CO（2）拍摄。其中，在过去十年中，在许多应用中使用了包括金属 - 有机框架（MOF）和共价有机骨架（COF）的网状材料，并且已成为CO 2的光电的先进催化平台。此进度报告旨在提供表征的基本原理，机制和方法，以了解CO（2）次拍摄过程中的洞察力。此外，该进度报告突出了使用网状材料作为CO（2）的光电荧光的先进催化剂的成果，并探讨了MOFS / COF的结构特征与其光催化性能的关系。基于对CO（2）次拍照的近距离材料的改进，机会和挑战的理解，讨论了该技术的未来前景，以指导设计更好的CO（2）减少光催化剂的令人兴奋的研究。

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