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Dendrites in Solid-State Batteries: Ion Transport Behavior, Advanced Characterization, and Interface Regulation

机译：固态电池中的树突：离子传输行为，高级表征和接口调节

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摘要

Solid-state electrolytes (SSEs) are attracting growing interest for next-generation Li-metal batteries with theoretically high energy density, but they currently suffer from safety concerns caused by dendrite growth, hindering their commercial applications. Interfaces between SSEs and solid lithium are argued to be crucial, affecting dendrite growth and determining solid-state batteries (SSBs) performance. The buried and localized nature of the interface poses a huge challenge for direct characterization under working conditions. Recent review articles have been devoted to evaluating the conductivity and chemical stability of SSEs. Recognizing this, in this Review, the focus is on understanding lithium dendrite beyond conventional factors and offering a perspective on various surface/interface and microstructural phenomena that require close attention by both experimentalists and theoreticians. The complicated ion-transport mechanism and chemomechanical information correlated with interface and lithium dendrite are discussed. Rational solutions are provided to engineer functional interfaces to suppress lithium dendrites and accelerate progress towards the commercialization of SSBs.
机译：固态电解质（小规模企业）正吸引着理论上具有高能量密度的新一代锂金属电池越来越大的兴趣，但他们从目前造成枝晶生长的安全问题受到影响，阻碍了他们的商业应用。的SSE和固体锂之间接口认为是至关重要的，影响枝晶生长并确定固态电池（单链断裂）的性能。界面的埋藏和局部性质对直接表征的工作条件下，一个巨大的挑战。最近的评论文章一直致力于评估SSE的导电性和化学稳定性。认识到这一点，在此回顾，重点是理解锂枝晶超越常规因素，并提供对由两个实验者和理论家需要密切关注各种表面/界面和微观现象的立体图。复杂的离子传输机制和化学机械信息与接口相关和锂枝晶进行了讨论。提供合理的解决方案来设计功能接口来抑制锂枝晶，并加快实现办学团体的商业化进程。

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  • 来源
    《Advanced energy materials》 |2021年第18期|2003250.1-2003250.25|共25页
  • 作者

    Yu Zhenjiang; Zhang Xueyan; Fu Chuankai; Wang Han; Chen Ming; Yin Geping; Huo Hua; Wang Jiajun;

  • 作者单位

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

    Harbin Inst Technol Sch Chem & Chem Engn MIIT Key Lab Crit Mat Technol New Energy Convers Harbin 150001 Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
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  • 关键词

    advanced characterization; dendrites; interface; ion#8208; transport mechanism; solid#8208; state batteries;

    机译：先进的表征;枝形;界面;离子＆＃8208;运输机制;实体＆＃8208;国家电池;

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