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Aqueous Rechargeable Multivalent Metal-Ion Batteries: Advances and Challenges

机译：可充电的多价金属离子电池：进步和挑战

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摘要

Aqueous rechargeable multivalent metal-ion batteries (ARMMBs) have a great potential to meet the future demands in the wide spectrum of energy storage applications, ranging from wearables/portables to large-scale stationary energy storage. This is owing to the abundance of the electrode materials, their eco-friendliness, high safety, fast-charging capability, high power density, and long-cycling capability. There has been considerable progress in ARMMBs over the past ten years. However, their rather narrow operating voltage window and insufficient energy density are still the main barriers to their use as alternative power sources to replace the widely used lithium-ion batteries. In this overview, the key advantages and current challenges for ARMMBs with respect to the cathode materials, electrolytes, metal anodes, and their integrations into full cells are first examined. The recent approaches in addressing these key challenges are then looked into, focusing on the new designs of advanced electrode materials, electrolytes, and also their interfaces. Finally, perspectives on the near-future development of ARMMBs are presented, together with a brief roadmap, where one of main pursuits will be to translate ARMMBs from current laboratory prototypes to commercialization/industrialization.
机译：可充电的多价金属离子电池（ARMMBS）具有巨大的潜力，可以满足宽谱的能量存储应用中未来的需求，从可穿戴设备/便携包括大规模固定储能。这是由于电极材料的丰富，它们的生态友好性，高安全性，快速充电能力，高功率密度和长循环能力。过去十年，武装中有相当大的进展。然而，它们相当窄的工作电压窗口和能量密度不足仍然是它们用作替代电源的主要障碍，以更换广泛使用的锂离子电池。在这一概述中，首先检查了相对于阴极材料，电解质，金属阳极和它们对全细胞的整合臂的关键优势和电流挑战。然后调查最近解决这些关键挑战的方法，专注于先进电极材料，电解质以及它们的界面的新设计。最后，对ARMMBS的近期发展的观点以及一个简短的路线图，其中主要追求之一将转换从现有的实验室原型转换为商业化/工业化。

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