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Beyond Seashells: Bioinspired 2D Photonic and Photoelectronic Devices

机译:超越贝壳:受生物启发的2D光子和光电设备

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摘要

The discovery of novel materials that possess extraordinary optical properties are of special interest, as they inspire systems for next-generation solar energy harvesting and conversion devices. Learning from nature has inspired the development of many photonic nanomaterials with fascinating structural colors. 2D photonic nanostructures, inspired by the attractive optical properties found on the inner surfaces of seashells, are fabricated in a facile and scalable way. The shells generate shining clusters for preying on phototactic creatures through interaction with incident solar light in water. By alternately depositing graphene and 2D ultrathin TiO2 nanosheets to form 2D-2D heterostructures and homostructures, seashell-inspired nanomaterials with well-controlled parameters are successfully achieved. They exhibit exceptional interlayer charge transfer properties and ultrafast in-plane electron mobility and present fascinating nacre-mimicking optical properties and significantly enhanced light-response behavior when acting as photoelectrodes. A window into the fabrication of novel 2D photonic structures and devices is opened, paving the way for the design of high-performance solar-energy harvesting and conversion devices.
机译:具有非凡光学特性的新型材料的发现特别令人感兴趣,因为它们启发了下一代太阳能收集和转换设备的系统。向自然学习启发了许多具有迷人结构颜色的光子纳米材料的发展。二维光子纳米结构的灵感来自于贝壳内表面具有吸引力的光学特性,并且以一种简便且可扩展的方式制造。贝壳通过与水中入射的太阳光相互作用,生成闪亮的簇,以捕食光战术生物。通过交替沉积石墨烯和2D超薄TiO2纳米片以形成2D-2D异质结构和同质结构,可以成功获得具有良好参数控制的贝壳启发性纳米材料。它们具有出色的层间电荷转移性能和超快的面内电子迁移率,并具有令人着迷的珍珠质模仿光学性能,并在充当光电极时具有显着增强的光响应性能。打开了新颖的2D光子结构和器件制造的窗口,为高性能太阳能收集和转换设备的设计铺平了道路。

著录项

  • 来源
    《Advanced Functional Materials》 |2019年第29期|1901460.1-1901460.9|共9页
  • 作者单位

    Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4000, Australia;

    Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4000, Australia;

    Shanghai Univ, Inst Mat, Shanghai 200444, Peoples R China|Shanghai Univ, Inst Sustainable Energy, Shanghai 200444, Peoples R China;

    Jiangsu Univ Sci & Technol, Sch Mat Sci & Engn, Zhenjiang 212003, Jiangsu, Peoples R China;

    Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4000, Australia|CSIRO QUT Joint Sustainable Proc & Devices Lab, POB 218, Lindfield, NSW 2070, Australia;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    2D nanomaterials; bio-inspired materials; optoelectronic devices; photonic structures;

    机译:二维纳米材料;生物启发材料;光电器件;光子结构;

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