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Circumventing Wear and Tear of Adaptive Porous Materials

机译：规避自适应多孔材料的磨损

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The assessment of the architectural stability of molecular porous materials is not yet a common practice, but critical to their understanding and development. The conformational adaptation of porous materials to guest binding and other chemical dynamics poses a risk of architectural damage, leading to performance deterioration during their prolonged usage. The deformation of the framework backbone and the disconnection of building units are driven by chemical, mechanical, and thermal perturbations, and can be quantitatively described by the term connection completeness. Analytical means that can be used to measure this parameter are presented in order to provide a standard, practical protocol for evaluating architectural damage made to framework materials. Preventive and remedial strategies are proposed for enhancing the architectural integrity of frameworks without compromising their functional mechanisms, paving the way to the design of robust yet adaptive materials. In this way, the discussion on architectural stability is initiated, and readers are encouraged to carefully characterize molecular porous materials for a better understanding of their structure-property relationship.
机译：对分子多孔材料的建筑稳定性的评估尚未成为常见的做法，对他们的理解和发展至关重要。多孔材料对客户约束和其他化学动力学的构象适应构建建筑损伤的风险，导致其延长使用过程中的性能恶化。框架骨架的变形和建筑物单元的断开由化学，机械和热扰动驱动，并且可以通过术语连接完整性定量描述。提供可用于测量该参数的分析装置，以提供用于评估对框架材料所做的架构损坏的标准实用方案。提出了提高框架架构完整性的预防性和补救策略，而不会影响其功能机制，铺平了稳健的自适应材料的设计。以这种方式，启动了关于建筑稳定性的讨论，并鼓励读者仔细描述分子多孔材料以更好地了解其结构性质关系。

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