Polymer-Based Solid Electrolytes: Material Selection, Design, and Application

Xi Guan; Xiao Min; Wang Shuanjin; Han Dongmei; Li Yuning; Meng Yuezhong

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Polymer-Based Solid Electrolytes: Material Selection, Design, and Application

机译：基于聚合物的固体电解质：材料选择，设计和应用

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Polymer-based solid electrolytes (PSEs) have attracted tremendous interests for the next-generation lithium batteries in terms of high safety and energy density along with good flexibility. Remarkable performances have been demonstrated in PSEs, which endowed PSEs with the potential to replace liquid electrolytes to meet the market demands. In this review, polymer matrices, different polymer architectures, and functional filler materials used in PSEs are discussed to explore the design concepts, methodologies, working mechanisms, and pros and cons of various PSEs. In addition, their recent notable applications in all-solid-state lithium ion batteries, lithium-sulfur batteries, suppression of lithium dendrites, and flexible lithium batteries are also introduced. Finally, the challenges and future prospects are sketched to provide strategies to explore novel PSEs for high-performance all-solid-state lithium batteries.

机译：基于聚合物的固体电解质（PSES）在高安全性和能量密度方面吸引了下一代锂电池的巨大兴趣，以及良好的灵活性。 PSE中已经证明了显着的表演，其赋予PSE具有替代液体电解质以满足市场需求的潜力。在本次综述中，讨论了聚合物基质，不同的聚合物架构和PSE中使用的功能填料材料，以探索各种PSE的设计概念，方法，工作机制和利弊。此外，还引入了全固态锂离子电池，锂 - 硫磺电池，锂树突抑制和柔性锂电池中的最近显着的应用。最后，勾勒出挑战和未来的前景，为探索高性能全固态锂电池的新型PSES提供策略。

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来源
《Advanced Functional Materials》 |2021年第9期|2007598.1-2007598.28|共28页
作者
Xi Guan; Xiao Min; Wang Shuanjin; Han Dongmei; Li Yuning; Meng Yuezhong;
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Sun Yat Sen Univ Sch Mat Sci & Engn State Key Lab Optoelect Mat & Technol Key Lab Low Carbon Chem & Energy Conservat Guangd Guangzhou 510275 Peoples R China|Univ Waterloo Dept Chem Engn 200 Univ Ave West Waterloo ON N2L 3G1 Canada|Univ Waterloo Waterloo Inst Nanotechnol WIN 200 Univ Ave West Waterloo ON N2L 3G1 Canada;

Sun Yat Sen Univ Sch Mat Sci & Engn State Key Lab Optoelect Mat & Technol Key Lab Low Carbon Chem & Energy Conservat Guangd Guangzhou 510275 Peoples R China;

Sun Yat Sen Univ Sch Mat Sci & Engn State Key Lab Optoelect Mat & Technol Key Lab Low Carbon Chem & Energy Conservat Guangd Guangzhou 510275 Peoples R China;

Sun Yat Sen Univ Sch Mat Sci & Engn State Key Lab Optoelect Mat & Technol Key Lab Low Carbon Chem & Energy Conservat Guangd Guangzhou 510275 Peoples R China;

Univ Waterloo Dept Chem Engn 200 Univ Ave West Waterloo ON N2L 3G1 Canada|Univ Waterloo Waterloo Inst Nanotechnol WIN 200 Univ Ave West Waterloo ON N2L 3G1 Canada;

Sun Yat Sen Univ Sch Mat Sci & Engn State Key Lab Optoelect Mat & Technol Key Lab Low Carbon Chem & Energy Conservat Guangd Guangzhou 510275 Peoples R China;

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正文语种 eng
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关键词
composite electrolytes; lithium battery; polymer electrolytes; solid state battery;

机译：复合电解质;锂电池;聚合物电解质;固态电池;

Polymer-Based Solid Electrolytes: Material Selection, Design, and Application

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