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Frontiers in the Growth of Complex Oxide Thin Films: Past, Present, and Future of Hybrid MBE

机译:复合氧化物薄膜生长的前沿领域:混合MBE的过去,现在和未来

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摘要

Driven by an ever-expanding interest in new material systems with new functionality, the growth of atomic-scale electronic materials by molecular beam epitaxy (MBE) has evolved continuously since the 1950s. Here, a new MBE technique called hybrid-MBE (hMBE) is reviewed that has been proven a power-ful approach for tackling the challenge of growing high-quality, multi-component complex oxides, specifically the ABO(3) perovskites. The goal of this work is to (1) discuss the development of hMBE in a historical context, (2) review the advantageous surface kinetics and chemistry that enable the self-regulated growth of ABO(3) perovskites, (3) layout the key components and technical challenges associated with hMBE, (4) review the status of the field and the materials that have been successfully grown by hMBE which demonstrate its general applicability, and (5) discuss the future of hMBE in regards to technical innovations and expansion into new material classes, which are aimed at expanding into industrial realm and at tackling new scientific endeavors.%1702772.1-1702772.41
机译:自从对具有新功能的新材料系统不断增长的兴趣驱使,自1950年代以来,分子束外延(MBE)促进了原子级电子材料的发展。在这里,对一种新的称为混合MBE(hMBE)的MBE技术进行了综述,该技术已被证明是解决日益增长的高质量,多组分复合氧化物(特别是ABO(3)钙钛矿)挑战的强大方法。这项工作的目的是(1)在历史背景下讨论hMBE的发展;(2)审查有利的表面动力学和化学性质,使ABO(3)钙钛矿能够自我调节生长;(3)布置关键与hMBE相关的组件和技术挑战,(4)回顾该领域的现状以及hMBE成功开发的材料,以证明其具有普遍的适用性,并且(5)讨论hMBE在技术创新和扩展方面的未来新材料类,旨在扩展到工业领域并应对新的科学工作。%1702772.1-1702772.41

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