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首页> 外文期刊>Advanced Functional Materials >Fully Solution-Processed Small Molecule Semitransparent Solar Cells: Optimization of Transparent Cathode Architecture and Four Absorbing Layers
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Fully Solution-Processed Small Molecule Semitransparent Solar Cells: Optimization of Transparent Cathode Architecture and Four Absorbing Layers

机译：完全溶液处理的小分子半透明太阳能电池：透明阴极体系结构和四个吸收层的优化

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摘要

Semitransparent solar cells (SSCs) can open photovoltaic applications in many commercial areas, such as power-generating windows and building integrated photovoltaics. This study successfully demonstrates solution-processed small molecule SSCs with a conventional configuration for the presently tested material systems, namely BDTT-S-TR:PC70BM, N(Ph-2T-DCN-Et)(3):PC70BM, SMPV1:PC70BM, and UU07:PC60BM. The top transparent cathode coated through solution processes employs a highly transparent silver nanowire as electrode together with a combination interface bilayer of zinc oxide nanoparticles (ZnO) and a perylene diimide derivative (PDINO). This ZnO/PDINO bilayer not only serves as an effective cathode buffer layer but also acts as a protective film on top of the active layer. With this integrated contribution, this study achieves a power conversion efficiency (PCE) of 3.62% for fully solution-processed SSCs based on BDTT-S-TR system. Furthermore, the other three systems with various colors exhibited the PCEs close to 3% as expected from simulations, demonstrate the practicality and versatility of this printed semitransparent device architecture for small molecule systems. This work amplifies the potential of small molecule solar cells for window integration.
机译：半透明太阳能电池（SSC）可以在许多商业领域中打开光伏应用，例如发电窗口和建筑集成光伏。这项研究成功地证明了经溶液处理的小分子SSC，具有用于当前测试材料系统的常规配置，即BDTT-S-TR：PC70BM，N（Ph-2T-DCN-Et）（3）：PC70BM，SMPV1：PC70BM，和UU07：PC60BM。通过溶液工艺涂覆的顶部透明阴极采用高度透明的银纳米线作为电极，以及氧化锌纳米颗粒（ZnO）和a二酰亚胺衍生物（PDINO）的组合界面双层。 ZnO / PDINO双层膜不仅可以用作有效的阴极缓冲层，还可以用作有源层顶部的保护膜。借助这一综合贡献，本研究对于基于BDTT-S-TR系统的完全溶液处理的SSC，实现了3.62％的功率转换效率（PCE）。此外，其他三种具有各种颜色的系统显示的PCE接近仿真所期望的3％，证明了这种印刷的半透明器件体系结构用于小分子系统的实用性和多功能性。这项工作扩大了小分子太阳能电池进行窗集成的潜力。

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  • 来源
    《Advanced Functional Materials》 |2016年第25期|4543-4550|共8页
  • 作者

    Min Jie; Bronnbauer Carina; Zhang Zhi-Guo; Cui Chaohua; Luponosov Yuriy N.; Ata Ibrahim; Schweizer Peter; Przybilla Thomas; Guo Fei; Ameri Tayebeh; Forberich Karen; Spiecker Erdmann; Baeuerle Peter; Ponomarenko Sergei A.; Li Yongfang; Brabec Christoph J.;

  • 作者单位

    Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol I MEET, Martensstr 7, D-91058 Erlangen, Germany;

    Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol I MEET, Martensstr 7, D-91058 Erlangen, Germany|Erlangen Grad Sch Adv Opt Technol SAOT, Paul Gordan Str 6, D-91052 Erlangen, Germany;

    Chinese Acad Sci, Inst Chem, CAS Key Lab Organ Solids, Beijing 100190, Peoples R China;

    Soochow Univ, Coll Chem Chem Engn & Mat Sci, Lab Adv Optoelect Mat, Suzhou 215123, Peoples R China;

    Russian Acad Sci, Enikolopov Inst Synthet Polymer Mat, Profsoyuznaya St 70, Moscow 117393, Russia;

    Univ Ulm, Inst Organ Chem & Adv Mat 2, Albert Einstein Allee 11, D-89081 Ulm, Germany;

    Univ Erlangen Nurnberg, Ctr Nanoanal & Electron Microscopy, Cauerstr 6, D-91058 Erlangen, Germany;

    Univ Erlangen Nurnberg, Ctr Nanoanal & Electron Microscopy, Cauerstr 6, D-91058 Erlangen, Germany;

    Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol I MEET, Martensstr 7, D-91058 Erlangen, Germany;

    Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol I MEET, Martensstr 7, D-91058 Erlangen, Germany;

    Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol I MEET, Martensstr 7, D-91058 Erlangen, Germany;

    Univ Ulm, Inst Organ Chem & Adv Mat 2, Albert Einstein Allee 11, D-89081 Ulm, Germany|Univ Erlangen Nurnberg, Ctr Nanoanal & Electron Microscopy, Cauerstr 6, D-91058 Erlangen, Germany;

    Russian Acad Sci, Enikolopov Inst Synthet Polymer Mat, Profsoyuznaya St 70, Moscow 117393, Russia|Moscow MV Lomonosov State Univ, Dept Chem, Leninskie Gory 1-3, Moscow 119991, Russia;

    Chinese Acad Sci, Inst Chem, CAS Key Lab Organ Solids, Beijing 100190, Peoples R China|Soochow Univ, Coll Chem Chem Engn & Mat Sci, Lab Adv Optoelect Mat, Suzhou 215123, Peoples R China;

    Univ Erlangen Nurnberg, Inst Mat Elect & Energy Technol I MEET, Martensstr 7, D-91058 Erlangen, Germany|Bavarian Ctr Appl Energy Res ZAE Bayern, Haberstr 2a, D-91058 Erlangen, Germany;

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  • 正文语种 eng
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  • 关键词

    semitransparent solar cells; building integrated photovoltaics; small molecule; interface bilayer; power conversion efficiency;

    机译：半透明太阳能电池;建筑集成光伏;小分子;界面双层;功率转换效率;

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