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Tough Hydrogels with Programmable and Complex Shape Deformations by Ion Dip-Dyeing and Transfer Printing

机译:通过离子浸染和转移印刷具有可编程和复杂形状变形的坚韧水凝胶

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摘要

Stimuli-responsive hydrogels with high mechanical strength, programmable deformation, and simple preparation are essential for their practical applications. Here the preparation of tough hydrogels with programmable and complex shape deformations is reported. Janus hydrogels with different compositions and hydrophilic natures on the two surfaces are first prepared, and they exhibit reversible bending/unbending upon swelling/deswelling processes. More impressively, the deformation rate and extent of the hydrogels can further be easily controlled through an extremely simple and versatile ion dip-dyeing (IDD) and/or ion transfer printing (ITP) method. By selectively printing proper patterns on 1D gel strips, 2D gel sheets and 3D gel structures, the transformations from 1D to 2D, 2D to 3D, and 3D to more complicated 3D shapes can be achieved after swelling the ion-patterned hydrogels in water. The swelling-deformable Janus and ion-patterned hydrogels with high mechanical strengths and programmable deformations can find many practical applications, such as soft machines.
机译:具有高机械强度,可编程变形和简单制备的刺激响应水凝胶对于其实际应用至关重要。此处报道了具有可编程和复杂形状变形的坚韧水凝胶的制备。首先制备在两个表面上具有不同组成和亲水性质的Janus水凝胶,并且它们在溶胀/溶胀过程中表现出可逆的弯曲/未弯曲。更令人印象深刻的是,水凝胶的变形速率和程度可以通过极其简单和通用的离子浸染(IDD)和/或离子转移印刷(ITP)方法轻松控制。通过在水中溶胀离子图案化的水凝胶后,通过在1D凝胶条,2D凝胶片和3D凝胶结构上选择性地打印适当的图案,可以实现从1D到2D,2D到3D和3D到更复杂的3D形状的转变。具有高机械强度和可编程变形的可溶胀变形的Janus和离子模式水凝胶可以找到许多实际应用,例如软机。

著录项

  • 来源
    《Advanced Functional Materials》 |2016年第25期|4491-4500|共10页
  • 作者单位

    Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China;

    Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China;

    Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China;

    Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China;

    Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China;

    Beijing Normal Univ, Coll Chem, Beijing Key Lab Energy Convers & Storage Mat, Beijing 100875, Peoples R China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    actuators; hydrogels; ion dip-dyeing; ion transfer printing; stimuli-responsive materials;

    机译:促动器;水凝胶;离子浸染;离子转移印刷;刺激响应材料;

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