Concentration Polarization of Salt-Containing Liquid Electrolytes

Joachim Maier

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Concentration Polarization of Salt-Containing Liquid Electrolytes

机译：含盐液体电解质的浓度极化

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Using the example of Li-battery electrolytes, the importance of the concept of conservative ensembles for polarization behavior and transference measurements of salt-containing liquid electrolytes is stressed. The conventional evaluation of the stationary values fails if the ion pair is mobile and can act as a vehicle of a single ion such as Li~+. The necessary generalization is considered. While the analytical form of the time dependence of voltage or current is not affected provided the ion pairing is sufficiently fast, the diffusion coefficient contains nontrivial extra contributions. Finally, soggy-sand electrolytes are inspected, in which polarization occurs in the space-charge zones.

机译：以锂电池电解质为例，强调了保守集合概念对含盐液体电解质的极化行为和迁移率测量的重要性。如果离子对是可移动的并且可以充当单个离子（例如Li〜+）的媒介，则固定值的常规评估将失败。考虑必要的概括。只要离子对足够快，电压或电流与时间的关系的分析形式就不会受到影响，但是扩散系数包含了非常重要的额外贡献。最后，检查湿沙电解质，其中极化发生在空间电荷区。

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《Advanced Functional Materials》 |2011年第8期|p.1448-1455|共8页
作者
Joachim Maier;
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Max Planck Institutfur Festkorperforschung Heisenbergstrasse 1, Stuttgart 70569, Germany;

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Concentration Polarization of Salt-Containing Liquid Electrolytes

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