Efficient Metal-Free Electrocatalysts from N-Doped Carbon Nanomaterials: Mono-Doping and Co-Doping

Gao Kun; Wang Bin; Tao Li; Cunning Benjamin V; Zhang Zhipan; Wang Shuangyin; Ruoff Rodney S.; Qu Liangti

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Efficient Metal-Free Electrocatalysts from N-Doped Carbon Nanomaterials: Mono-Doping and Co-Doping

机译：N掺杂碳纳米材料的高效无金属电催化剂：单掺杂和共掺杂

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摘要

N-doped carbon nanomaterials have rapidly grown as the most important metal-free catalysts in a wide range of chemical and electrochemical reactions. This current report summarizes the latest advances in N-doped carbon electrocatalysts prepared by N mono-doping and co-doping with other heteroatoms. The structure-performance relationship of these materials is subsequently rationalized and perspectives on developing more efficient and sustainable electrocatalysts from carbon nanomaterials are also suggested.

机译：氮掺杂的碳纳米材料已迅速发展成为广泛的化学和电化学反应中最重要的无金属催化剂。本报告总结了通过单掺杂N和与其他杂原子共掺杂制备的N掺杂碳电催化剂的最新进展。随后合理化了这些材料的结构-性能关系，并提出了从碳纳米材料开发更高效和可持续的电催化剂的观点。

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来源
《Advanced Materials》 |2019年第13期|1805121.1-1805121.11|共11页
作者
Gao Kun; Wang Bin; Tao Li; Cunning Benjamin V; Zhang Zhipan; Wang Shuangyin; Ruoff Rodney S.; Qu Liangti;
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作者单位

Beijing Inst Technol, Sch Chem & Chem Engn, Key Lab Photoelect Electrophoton Convers Mat, Key Lab Cluster Sci,Minist Educ China, Beijing 100081, Peoples R China;

Inst Basic Sci, CMCM, Ulsan 44919, South Korea;

Hunan Univ, State Key Lab Chem Biosensing & Chemometr, Prov Hunan Key Lab Graphene Mat & Devices, Coll Chem & Chem Engn, Changsha 410082, Hunan, Peoples R China;

Inst Basic Sci, CMCM, Ulsan 44919, South Korea;

Beijing Inst Technol, Sch Chem & Chem Engn, Key Lab Photoelect Electrophoton Convers Mat, Key Lab Cluster Sci,Minist Educ China, Beijing 100081, Peoples R China;

Hunan Univ, State Key Lab Chem Biosensing & Chemometr, Prov Hunan Key Lab Graphene Mat & Devices, Coll Chem & Chem Engn, Changsha 410082, Hunan, Peoples R China;

Inst Basic Sci, CMCM, Ulsan 44919, South Korea|Ulsan Natl Inst Sci & Technol, Dept Chem, Ulsan 44919, South Korea|Ulsan Natl Inst Sci & Technol, Sch Mat Sci & Engn, Ulsan 44919, South Korea;

Beijing Inst Technol, Sch Chem & Chem Engn, Key Lab Photoelect Electrophoton Convers Mat, Key Lab Cluster Sci,Minist Educ China, Beijing 100081, Peoples R China;

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正文语种 eng
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关键词
co-doping; electrocatalysts; metal-free; mono-doping; N-doped carbon;

机译：共掺杂;电催化剂;无金属;单掺杂;N掺杂碳;

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专利

1. 1D N-doped hierarchically porous hollow carbon tubes derived from a supramolecular template as metal-free electrocatalysts for a highly efficient oxygen reduction reaction [J] . Zhao Lei, Sui Xu-Lei, Zhou Qing-Yan, Journal of Materials Chemistry, A. Materials for energy and sustainability . 2018,第15期

机译：1D N掺杂的分层多孔中空碳管从超分子模板衍生，作为无金属电催化剂，用于高效的氧还原反应
2. Metal-Free Artificial Photosynthesis of Carbon MonoxidernUsing N-Doped ZnTe Nanorod Photocathode Decorated with N-Doped Carbon Electrocatalyst Layer [J] . Jang Youn Jeong, Bhatt Mahesh Datt, Lee Jaehyuk, Advanced energy materials . 2018,第20期

机译：氮掺杂碳电催化剂层修饰的氮掺杂ZnTe纳米棒光阴极的无金属人工光合作用
3. Vertically Aligned BCN Nanotubes as Efficient Metal-Free Electrocatalysts for the Oxygen Reduction Reaction: A Synergetic Effect by Co-Doping with Boron and Nitrogen [J] . Shuangyin Wang, Eswaramoorthi Iyyamperumal, Ajit Roy Angewandte Chemie . 2011,第49期

机译：垂直排列的BCN纳米管作为高效的无金属氧还原反应的电催化剂：硼和氮共掺杂的协同效应
4. (Invited) Boron and Nitrogen Co-Doped Porous Carbon Nanofibers As Metal-Free Electrocatalysts for Highly Efficient Ammonia Electrosynthesis [C] . Yang Hou, Yan Kong Meeting of the Electrochemical Society;International Meeting on Chemical Sensors . 2020

机译：（邀请）硼和氮掺杂多孔碳纳米纤维作为无金属电催化剂，用于高效氨电催化剂
5. Metal-free Electrocatalysts for Oxygen Evolution Reaction and Photocatalysts for Carbon Dioxide Reduction Reaction [D] . Kadel, Usha Pandey. 2018

机译：用于氧气进化反应的无金属电催化剂和用于二氧化碳还原反应的光催化剂
6. Identification of catalytic sites for oxygen reduction and oxygen evolution in N-doped graphene materials: Development of highly efficient metal-free bifunctional electrocatalyst [O] . Hong Bin Yang, Jianwei Miao, Sung-Fu Hung, 2016

机译：鉴定氮掺杂石墨烯材料中用于氧还原和氧释放的催化位点：高效无金属双功能电催化剂的开发
7. N-Doped Porous Carbon from Sargassum spp. as Efficient Metal-Free Electrocatalysts for O2 Reduction in Alkaline Fuel Cells [O] . K. Pérez-Salcedo, Xuan Shi, Arunachala Kannan, 2019

机译：来自Sargassum SPP的N掺杂多孔碳。作为碱性燃料电池O2减少的高效无金属电催化剂

Efficient Metal-Free Electrocatalysts from N-Doped Carbon Nanomaterials: Mono-Doping and Co-Doping

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