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Graphene Nanoarchitectonics: Recent Advances in Graphene-Based Electrocatalysts for Hydrogen Evolution Reaction

机译:石墨烯纳米结构:氢发生反应的石墨烯基电催化剂的最新进展

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摘要

Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy-production and energy-consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene-based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene-based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed.
机译:在能源危机和环境污染的双重压力下,清洁和可再生能源氢的开发利用已成为可持续能源生产和能源消费系统发展的重要趋势。在这方面,电催化放氢反应(HER)为氢燃料的批量生产提供了有效和清洁的途径,并激发了可接受的成本的高活性HER电催化剂的设计和构建。特别地,基于石墨烯的电催化剂由于其独特的结构优点(包括大表面积,高电导率和良好的化学稳定性)而通常表现出增强的HER性能。考虑到过去几年中对该主题的快速增长的研究热情,本文对石墨烯基电催化剂的最新进展进行了综述,涵盖了各种先进的合成策略,微观结构表征以及此类材料在HER电催化中的应用。最后,提出并讨论了有关该新兴领域所面临的挑战和机遇的未来观点。

著录项

  • 来源
    《Advanced Materials》 |2019年第48期|1903415.1-1903415.34|共34页
  • 作者单位

    Hohai Univ Coll Mech & Mat Nanjing 210098 Jiangsu Peoples R China;

    Queensland Univ Technol Sch Chem Phys & Mech Engn 2 George St Brisbane Qld 4001 Australia;

    Hohai Univ State Key Lab Hydrol Water Resources & Hydraul En Nanjing 210098 Jiangsu Peoples R China;

    Tianjin Univ Inst Mol Plus 11 Bldg 92 Weijin Rd Tianjin 300072 Peoples R China|Univ Wollongong Australian Inst Innovat Mat Squires Way North Wollongong NSW 2500 Australia|Natl Inst Mat Sci Int Ctr Mat Nanoarchitecton WPI MANA 1-1 Namiki Tsukuba Ibaraki 3050044 Japan;

    Univ Queensland Sch Chem Engn Brisbane Qld 4072 Australia|Univ Queensland AIBN Brisbane Qld 4072 Australia|Kyung Hee Univ Dept Plant & Environm New Resources 1732 Deogyeong Daero Yongin 446701 Gyeonggi Do South Korea;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    electrocatalysts; graphene; hybrid structures; hydrogen evolution reaction; nanoparticles;

    机译:电催化剂;石墨烯混合结构;析氢反应纳米粒子;

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