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Conductive Silk-Based Composites Using Biobased Carbon Materials

机译：使用生物基碳材料的导电丝基复合材料

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摘要

There is great interest in developing conductive biomaterials for the manufacturing of sensors or flexible electronics with applications in healthcare, tracking human motion, or in situ strain measurements. These biomaterials aim to overcome the mismatch in mechanical properties at the interface between typical rigid semiconductor sensors and soft, often uneven biological surfaces or tissues for in vivo and ex vivo applications. Here, the use of biobased carbons to fabricate conductive, highly stretchable, flexible, and biocompatible silk-based composite biomaterials is demonstrated. Biobased carbons are synthesized via hydrothermal processing, an aqueous thermochemical method that converts biomass into a carbonaceous material that can be applied upon activation as conductive filler in composite biomaterials. Experimental synthesis and full-atomistic molecular dynamics modeling are combined to synthesize and characterize these conductive composite biomaterials, made entirely from renewable sources and with promising applications in fields like biomedicine, energy, and electronics.
机译：开发用于制造传感器或柔性电子器件的导电生物材料引起了人们极大的兴趣，这些导电材料用于医疗保健，跟踪人体运动或原位应变测量。这些生物材料旨在克服用于体内和离体应用的典型刚性半导体传感器与柔软，通常不平坦的生物表面或组织之间的界面处机械性能的失配。在此，证明了使用生物基碳来制造导电的，高度可拉伸的，柔性的和生物相容的丝基复合生物材料。生物基碳是通过水热处理工艺合成的，该工艺是一种水热化学方法，可将生物质转化为碳质材料，可在活化后用作复合生物材料中的导电填料。实验合成和全原子分子动力学建模相结合，以合成和表征这些导电复合生物材料，这些材料完全由可再生资源制成，并在生物医学，能源和电子学等领域具有广阔的应用前景。

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