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Supramolecular-Macrocycle-Based Crystalline Organic Materials

机译：超分子 - 大环基结晶有机材料

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摘要

Abstract Supramolecular macrocycles are well known as guest receptors in supramolecular chemistry, especially host−guest chemistry. In addition to their wide applications in host−guest chemistry and related areas, macrocycles have also been employed to construct crystalline organic materials (COMs) owing to their particular structures that combine both rigidity and adaptivity. There are two main types of supramolecular‐macrocycle‐based COMs: those constructed from macrocycles themselves and those prepared from macrocycles with other organic linkers. This review summarizes recent developments in supramolecular‐macrocycle‐based COMs, which are categorized by various types of macrocycles, including cyclodextrins, calixarenes, resorcinarenes, pyrogalloarenes, cucurbiturils, pillararenes, and others. Effort is made to focus on the structures of supramolecular‐macrocycle‐based COMs and their structure–function relationships. In addition, the application of supramolecular‐macrocycle‐based COMs in gas storage or separation, molecular separation, solid‐state electrolytes, proton conduction, iodine capture, water or environmental treatment, etc., are also presented. Finally, perspectives and future challenges in the field of supramolecular‐macrocycle‐based COMs are discussed.
机译：摘要超分子宏ycles是众所周知的超分子化学，特别是宿主化学。除了在宿主 - 客体化学和相关领域的广泛应用外，还被用于构建刚性结构的宏型有机材料（COMS），其特定的结构结合了刚性和适应性。基于超分子 - 大环的COMS有两种主要类型：由宏细胞本身构成的那些，并用其他有机接头用宏杂种制备的那些。本综述总结了基于Supramular-Macrocycle的COMS的最新发展，其被各种类型的宏杂种分类，包括环糊精，钙屈剂，间苯二酚，过热剂，葫芦菌，氨基酮，丘脂等。努力专注于基于超分子 - 宏系的COM的结构及其结构功能关系。此外，还还提出了在气体储存或分离，分子分离，固态电解质，质子传导，水或环境处理等中施加超分子 - 大环基COM的应用。最后，讨论了基于超分子 - 宏循环的COMS领域的观点和未来挑战。

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