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Energy analyses and process integration of coal-fired power plant with CO_2 capture using sodium-based dry sorbents

机译:使用钠基干吸附剂进行CO_2捕集的燃煤电厂的能量分析和过程集成

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摘要

Post-combustion CO2 capture using sodium-based solid sorbents is viewed as a promising technology owing to its advantages of low cost, easy accessibility, and low desorption temperature. It is necessary to evaluate the efficiency penalty of coal-fired power plants (CFPPs) using sodium-based solid sorbents prior to industrial applications. In this study, a typical 300MW CFPP, coupled with a sodium-based CO2 capture system, was established in Aspen Plus. The simulation results demonstrate that the gross efficiency penalty was 15.5% as a result of this process. The energy consumption for the CO2 capture process was 7.23 GJ/tCO(2) without any heat recovery; substantially higher than that of typical Monoethanolamine (MEA)-based CCS technologies, which is in the range of 3.8 to 4.2 GJ/tCO(2). By recovering the heat of the outlet gas and sorbents from the desorption reactor, the energy consumption was reduced to 4.04 GJ/tCO(2), with a gross efficiency penalty of 8.55%. To recover low-level heat from the sorption reactor, an economical system was proposed, consisting of a CFPP with CO2 capture and a cogeneration unit with an absorption heat pump. The energy consumption was further reduced to 1.08 GJ/tCO(2), and the net efficiency penalty of this economical system was 11.99%. This method may provide significant economic and application prospects for sodium-based CO2 capture technology.
机译:使用钠基固体吸附剂的燃烧后二氧化碳捕集由于其成本低,易于获得和解吸温度低等优点而被视为有前途的技术。在工业应用之前,有必要评估使用钠基固体吸附剂的燃煤电厂(CFPP)的效率损失。在这项研究中,在Aspen Plus中建立了典型的300MW CFPP以及基于钠的CO2捕集系统。仿真结果表明,该过程的总效率损失为15.5%。 CO2捕集过程的能耗为7.23 GJ / tCO(2),没有任何热量回收。大大高于基于单乙醇胺(MEA)的典型CCS技术(在3.8至4.2 GJ / tCO(2)范围内)。通过从解吸反应器中回收出口气体和吸附剂的热量,能量消耗降低至4.04 GJ / tCO(2),总效率损失为8.55%。为了从吸附反应器中回收少量热量,提出了一种经济的系统,该系统由具有CO2捕集功能的CFPP和带有吸收式热泵的热电联产装置组成。能耗进一步降低至1.08 GJ / tCO(2),该经济系统的净效率损失为11.99%。该方法可为钠基二氧化碳捕集技术提供重要的经济和应用前景。

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