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The interaction effects between adsorbed molecules in the Statistical Rate Theory approach to the kinetics of mixed-gas adsorption

机译：统计速率理论方法中混合气体吸附动力学中吸附分子之间的相互作用

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摘要

Kinetics of adsorption of single gases and their binary mixture on an energetically homogeneous surface are studied theoretically using the Statistical Rate Theory (SRT) of interfacial transport. Additionally, the influence of intermolecular interactions on the rate of adsorption is modeled using the Regular Adsorbed Solution Theory. The theoretical results are classified and assigned to different types of experimental conditions under which the changes of the adsorbate concentration near the adsorbing surface are considerable or they are negligible. Predictions of the theory are verified using adsorption data measured in real systems.
机译：使用界面传输的统计速率理论（SRT），从理论上研究了单一气体及其二元混合物在能量均匀表面上的吸附动力学。另外，使用常规吸附溶液理论对分子间相互作用对吸附速率的影响进行建模。将理论结果分类并分配给不同类型的实验条件，在这些条件下，吸附表面附近的吸附物浓度变化相当大或可忽略不计。使用在实际系统中测量的吸附数据验证了该理论的预测。

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