We report interstellar Fe II and Si II column densities toward six translucent sight lines (A_V approx > 1) observed with the Space Telescope Imaging Spectrograph (STIS). The abundances were determined from the absorption of Si II] at 2335 A, and several weak Fe transitions including the first reported detections of the λ2234 line. We derive an empirical f-value for the FeII λ2234 transition of log (fλ) = -1.54 ± 0.05. The observed sight lines sample a variety of extinction characteristics as indicated by their R_V values, which range from 2.6 to 5.8. The dust-phase abundances of both Si and Fe are positively correlated with the small-grain population (effective radii smaller than a few hundred μm) toward the targets. The physical conditions along the sight lines suggest that this relationship may be due to differences in the survival of small particles in some interstellar environments. The chemical composition of the small grains could either resemble dust mantles or be silicate-rich.
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