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Trace gases in the atmosphere over Russian cities

机译:俄罗斯城市大气中的微量气体

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Multiyear observational data (obtained at the mobile railroad laboratory in the course of the 1995-2010 TROICA experiments) on the composition and state of the atmosphere were used to study the features of both spatial and temporal variations in the contents of trace gases in the surface air layer over Russian cities. The obtained characteristics of urban air noticeably differ from those obtained at stationary stations. The emission fluxes of NOx, CO, and CH4 and their integral emissions from large cities have been estimated on the basis of observational data obtained at the mobile laboratory. The values of these emission fluxes reflect the state of urban infrastructure. The integral urban emissions of CO depend on the city size and vary from 50 Gg yr(-1) for Yaroslavl to 130 Gg yr(-1) for Yekaterinburg. For most cities, they agree with the EDGAR v4.2 data within the limits of experimental error. The agreement is worse for the emissions of NOx. The EDGAR v4.2 data on the emissions of CH4 seem to be overestimated. (C) 2016 Elsevier Ltd. All rights reserved.
机译:使用多年的观测数据(在1995-2010年TROICA实验过程中在移动铁路实验室获得)来了解大气的组成和状态,以研究地表中痕量气体含量的时空变化特征俄罗斯城市上空的空气层。所获得的城市空气特征与固定站获得的特征明显不同。根据在流动实验室获得的观测数据,估算了大城市的NOx,CO和CH4排放通量及其整体排放。这些排放通量的值反映了城市基础设施的状况。城市中一氧化碳的整体排放量取决于城市规模,从雅罗斯拉夫尔的50 Gg yr(-1)到叶卡捷琳堡的130 Gg yr(-1)不等。对于大多数城市,他们在实验误差的范围内同意EDGAR v4.2数据。对于NOx的排放,该协议更糟。 EDGAR v4.2有关CH4排放的数据似乎被高估了。 (C)2016 Elsevier Ltd.保留所有权利。

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