Shock Tube and Modeling Study of Chemical lonization in the Oxidation of Acetylene and Methane Mixtures

Agafonov G. L.; Mikhailov D. I.; Smirnov V. N.; Tereza A. M.; Vlasov P. A.; Zhiltsova I. V.

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Shock Tube and Modeling Study of Chemical lonization in the Oxidation of Acetylene and Methane Mixtures

机译：乙炔和甲烷混合物氧化过程中的激波管和化学电离建模研究

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Chemical ionization during the oxidation of methane and acetylene is experimentally and theoretically studied behind reflected shock waves over a wide temperature range and atmospheric pressure. The results of experimental measurements of the concentration of free electrons by microwave interferometry and electric probe method during the oxidation of acetylene and methane behind reflected shock waves are presented. A detailed kinetic model of the process of chemical ionization was developed. The results of experimental measurements and kinetic simulations are in good qualitative and quantitative agreement. The kinetic model of chemical ionization makes it possible to improve the kinetic description of the experimentally measured time histories of free electrons for the hydrocarbons studied.

机译：在较宽的温度范围和大气压下，在反射的冲击波之后，对甲烷和乙炔氧化过程中的化学电离进行了实验和理论研究。给出了微波干涉法和电探针法在反射冲击波后乙炔和甲烷氧化过程中自由电子浓度的实验测量结果。建立了化学电离过程的详细动力学模型。实验测量和动力学模拟的结果在定性和定量方面吻合良好。化学电离的动力学模型可以改善所研究的烃类的自由电子的实验测量时间历史的动力学描述。

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来源
《Combustion Science and Technology》 |2016年第12期|1815-1830|共16页
作者
Agafonov G. L.; Mikhailov D. I.; Smirnov V. N.; Tereza A. M.; Vlasov P. A.; Zhiltsova I. V.;
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作者单位

Russian Acad Sci, Semenov Inst Chem Phys, Kosygin Str 4, Moscow 119991, Russia;

Natl Nucl Res Univ MEPHI, Minist Educ & Sci Russian Federat, Moscow, Russia;

Russian Acad Sci, Semenov Inst Chem Phys, Kosygin Str 4, Moscow 119991, Russia;

Russian Acad Sci, Semenov Inst Chem Phys, Kosygin Str 4, Moscow 119991, Russia;

Russian Acad Sci, Semenov Inst Chem Phys, Kosygin Str 4, Moscow 119991, Russia;

Russian Acad Sci, Semenov Inst Chem Phys, Kosygin Str 4, Moscow 119991, Russia;

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正文语种 eng
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关键词
Charged particles; Chemical ionization; Experimental data; Hydrocarbon oxidation; Kinetic simulations; Shock waves;

机译：带电粒子;化学电离;实验数据;烃类氧化;动力学模拟;冲击波;

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1. Chemical lonization of n-Hexane, Acetylene, and Methane behind Reflected Shock Waves [J] . Vlasov P. A., Zhiltsova I. V., Smirnov V. N., Combustion Science and Technology . 2018,第1a3期

机译：反射冲击波后正己烷，乙炔和甲烷的化学电离
2. Experimental and modeling study of shock-tube oxidation of acetylene [J] . Boris Eiteneer, Michael Frenklach International Journal of Chemical Kinetics . 2003,第9期

机译：乙炔激波管氧化的实验与模型研究
3. On initiation reactions of acetylene oxidation in shock tubes A quantum mechanical and kinetic modeling study [J] . Alexander Laskin, Hai Wang Chemical Physics Letters . 1999,第1a2期

机译：激波管中乙炔氧化引发反应的量子力学和动力学建模研究
4. Experimental and modelling study of gasoline surrogate mixtures oxidation in jet stirred reactor and shock tube [C] . M. Yahyaoui, N. Djebaieli-Chaumeix, P. Dagaut, International Symposium on Combustion; 20060805-11; University of Heidelberg(DE) . 2006

机译：喷射搅拌反应器和激波管中汽油替代混合物氧化的实验与模型研究
5. Interpretation of methane-ethane-acetylene-carbon monoxide correlations in atmospheric observations as constraints on sources of methane and chemical aging. [D] . Xiao, Yaping. 2007

机译：大气观测中甲烷-乙烷-乙炔-一氧化碳相关性的解释是对甲烷和化学老化源的限制。
6. A Shock Tube and Chemical Kinetic Modeling Study of the Oxidation of 25-Dimethylfuran [O] . Baptiste Sirjean, René Fournet, Pierre-Alexandre Glaude, -1

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7. Shock Tube and Chemical Kinetic Modeling Study of the Oxidation of 2,5-Dimethylfuran [O] . Sirjean, Baptiste, Fournet, René, Glaude, Pierre-Alexandre, 2013

机译：2,5-二甲基呋喃的氧化反应的激波管和化学动力学模型研究
8. Shock Tube Studies of Nitrogen Vibrational Relaxation and Methane Oxidation [R] . White, D. R. 1970

机译：氮振动弛豫和甲烷氧化的激波管研究

Shock Tube and Modeling Study of Chemical lonization in the Oxidation of Acetylene and Methane Mixtures

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