Singlet Oxygen Generation with Chemical Excitation of an Erythrosine–Luminol Conjugate

Nisa Yesilgul; T. Bilal Uyar; Ozlem Seven; Engin U. Akkaya

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Singlet Oxygen Generation with Chemical Excitation of an Erythrosine–Luminol Conjugate

机译：赤藓氨酸-鲁米诺偶联物的化学激发产生单线态氧

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Chemical generation of singlet oxygen under biologically relevant conditions is very important, considering the role played by singlet oxygen in cancer therapeutics. We now demonstrate that a luminol derivative can be chemically excited and transfer the excitation energy to the covalently attached photosensitizer derived from erythrosin. A photosensitizer module, when excited in this manner, can generate singlet oxygen in solution. As hydrogen peroxide is present in a relatively high concentration in cancer cells, singlet oxygen generation through chemical excitation may evolve into an important therapeutic approach.

机译：考虑到单线态氧在癌症治疗中的作用，在生物学相关条件下化学产生单线态氧非常重要。我们现在证明鲁米诺衍生物可以被化学激发并将激发能转移至衍生自赤藓红的共价连接的光敏剂。当以这种方式激发光敏剂模块时，它可以在溶液中产生单线态氧。由于过氧化氢以相对较高的浓度存在于癌细胞中，通过化学激发产生单线态氧可能演变成一种重要的治疗方法。

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《ACS Omega》 |2017年第4期|共5页
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Nisa Yesilgul; T. Bilal Uyar; Ozlem Seven; Engin U. Akkaya;
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1. X-ray induced singlet oxygen generation by nanoparticle-photosensitizer conjugates for photodynamic therapy: determination of singlet oxygen quantum yield [J] . Sandhya Clement, Wei Deng, Elizabeth Camilleri, Scientific reports. . 2016,第1期

机译：纳米粒子-光敏剂共轭物在X射线诱导的光动力疗法中产生单重态氧的产生：单重态氧量子产率的测定
2. Induction of benzo[a]pyrene Mono-oxygenase in liver cell culture by the photochemical generation of active oxygen species. Evidence for the involvement of singlet oxygen and the formation of a stable inducing intermediate [J] . A J Paine The biochemical journal . 1976,第1期

机译：通过光化学产生活性氧来诱导肝细胞培养物中的苯并[a] py单加氧酶。单线态氧参与并形成稳定的诱导中间体的证据
3. Induction of benzo[a]pyrene Mono-oxygenase in liver cell culture by the photochemical generation of active oxygen species. Evidence for the involvement of singlet oxygen and the formation of a stable inducing intermediate [J] . A J Paine The biochemical journal . 1976,第1期

机译：通过光化学产生活性氧来诱导肝细胞培养物中的苯并[a] py单加氧酶。单线态氧参与并形成稳定的诱导中间体的证据
4. Photochemical inactivation of viruses by antibody conjugates of compounds generating singlet oxygen [C] . Alexander P. Savitsky, Andrey I. Tourkin, Elena V. Tourkina, Conference on photodynamic therapy of cancer . 1994

机译：通过化合物的抗体缀合物产生的光化学灭活，生成单线氧的抗体缀合物
5. MECHANISMS OF PHOTOOXIDATIONS: ELECTRON-TRANSFER TO SINGLET OXYGEN, SUBSTRATE ENHANCED INTERSYSTEM CROSSING AS A SOURCE OF SINGLET OXYGEN AND SINGLET OXYGEN-OLEFIN INTERACTIONS. [D] . MANRING, LEWIS EDWARD. 1982

机译：光氧化的机理：电子转移到单氧，基质增强的系统间交叉作为单氧的来源和单氧-烯烃相互作用。
6. Singlet OxygenGeneration with Chemical Excitation of an Erythrosine–LuminolConjugate [O] . Nisa Yesilgul, T. Bilal Uyar, Ozlem Seven, 2017

机译：单线态氧化学激发产生赤藓氨酸-鲁米诺共轭
7. Singlet Oxygen Generation with Chemical Excitation of an Erythrosine–Luminol Conjugate [O] . Nisa Yesilgul, T. Bilal Uyar, Ozlem Seven, 2017

机译：用于化学激发赤藓红 - 鲁米诺共轭物的单线态氧生成
8. Chemical Generation and Deactivation of Oxygen Singlet Delta (Generation Chimique et Desactivation de l'Oxygene Singulet Delta). [R] . Barton, S. A. 1983

机译：氧单重态的化学生成和失活（生成Chimique和Desactivation de l'Oxygene singulet Delta）。

Singlet Oxygen Generation with Chemical Excitation of an Erythrosine–Luminol Conjugate

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