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A new indicator on the impact of large-scale circulation on wintertime particulate matter pollution over China

机译:大规模循环对中国冬季颗粒物污染影响的新指标

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Extreme particulate matter (PM) air pollution of January 2013 in China wasfound to be associated with an anomalous eastward extension of the SiberianHigh (SH). We developed a Siberian High position index (SHPI), which depictsthe mean longitudinal position of the SH, as a new indicator of thelarge-scale circulation pattern that controls wintertime air quality inChina. This SHPI explains 58 % (correlation coefficient of 0.76) of theinterannual variability of wintertime aerosol optical depth (AOD) retrievedby MODIS over North China (NC) during 2001–2013. By contrast, theintensity-based conventional Siberian High index (SHI) shows essentially noskill in predicting this AOD variability. On the monthly scale, somehigh-AOD months for NC are accompanied with extremely high SHPIs; notably,extreme PM pollution of January 2013 can be explained by the SHPI valueexceeding 2.6 times the standard deviation of the 2001–2013 January mean.When the SH extends eastward, thus higher SHPI, prevailing northwesterlywinds over NC are suppressed not only in the lower troposphere but also inthe middle troposphere, leading to reduced southward transport of pollutionfrom NC to South China (SC). The SHPI hence exhibits a significantlynegative correlation of ?0.82 with MODIS AOD over SC during 2001–2013,although the robustness of this correlation depends on that ofsatellite-derived AOD. The suppressed northwesterly winds during high-SHPIwinters also lead to increased relative humidity (RH) over NC. Both the windand RH changes are responsible for enhanced PM pollution over NC during thehigh-SHPI winters.
机译:发现2013年1月的中国极端颗粒物(PM)空气污染与西伯利亚高压(SH)向东异常延伸有关。我们开发了西伯利亚高空位置指数(SHPI),该指数描述了南半球的平均纵向位置,作为控制中国冬季空气质量的大规模循环模式的新指标。该SHPI解释了MODIS在华北地区(NC)在2001-2013年间获取的冬季气溶胶光学深度(AOD)的年际变化的58%(相关系数为0.76)。相比之下,基于强度的常规西伯利亚高指数(SHI)在预测这种AOD变异性时表现出本质的技巧。在月度范围内,NC的某些高AOD月份伴随着极高的SHPI。值得注意的是,2013年1月的极端PM污染可以通过SHPI值超过2001-2013年1月平均值的标准偏差的2.6倍来解释。当SH向东延伸时,因此SHPI较高,不仅在对流层低层,北半球的北风也受到抑制。而且在对流层中部,导致污染物从北向南向华南(SC)的向南运输减少。因此,在2001–2013年期间,SHPI与MODIS AOD的SC呈极显着负相关,约为0.82,尽管这种相关的鲁棒性取决于卫星衍生的AOD。在高SHPI冬季期间,西北风的抑制也导致了NC上相对湿度(RH)的增加。在高SHPI冬季,风和相对湿度的变化都导致NC上PM污染的增加。

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