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Observation of Poiseuille flow of phonons in black phosphorus

机译:黑磷中声子的泊肃叶流的观察

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The travel of heat in insulators is commonly pictured as a flow of phonons scattered along their individual trajectory. In rare circumstances, momentum-conserving collision events dominate, and thermal transport becomes hydrodynamic. One of these cases, dubbed the Poiseuille flow of phonons, can occur in a temperature window just below the peak temperature of thermal conductivity. We report on a study of heat flow in bulk black phosphorus between 0.1 and 80 K. We find a thermal conductivity showing a faster than cubic temperature dependence between 5 and 12 K. Consequently, the effective phonon mean free path shows a nonmonotonic temperature dependence at the onset of the ballistic regime, with a size-dependent Knudsen minimum. These are hallmarks of Poiseuille flow previously observed in a handful of solids. Comparing the phonon dispersion in black phosphorus and silicon, we show that the phase space for normal scattering events in black phosphorus is much larger. Our results imply that the most important requirement for the emergence of Poiseuille flow is the facility of momentum exchange between acoustic phonon branches. Proximity to a structural transition can be beneficial for the emergence of this behavior in clean systems, even when they do not exceed silicon in purity.
机译:绝缘子中的热传播通常被描绘为沿着其各自轨迹散布的声子流。在极少数情况下,保持动量的碰撞事件占主导,并且热传递变为流体动力学。其中一种情况被称为声子的Poiseuille流动,可能会在温度窗口内发生,该温度窗口正好位于导热系数的峰值温度以下。我们报告了一份关于散装黑磷在0.1和80 K之间的热流的研究报告。我们发现导热率显示出比立方温度在5和12 K之间更快的热导率。因此,有效声子平均自由程显示了一个非单调温度依赖性。弹道政权的爆发,其大小取决于克努森最小值。这些是以前在少数固体中观察到的泊瓦雪流的特征。比较声子在黑磷和硅中的色散,我们发现黑磷中正常散射事件的相空间要大得多。我们的结果表明,泊松尾流出现的最重要条件是声子声子分支之间动量交换的便利。即使在纯度不超过硅的情况下,接近结构转变也可能有益于在清洁系统中出现这种行为。

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