Carbon-containing bone hydroxyapatite obtained from tuna fish bone with high adsorption performance for Congo red

Qifan Peng; Fan Yu; Bicheng Huang; Yaqin Huang

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Carbon-containing bone hydroxyapatite obtained from tuna fish bone with high adsorption performance for Congo red

机译：从金枪鱼鱼骨中获得的对刚果红具有高吸附性能的含碳骨羟基磷灰石

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The carbon-containing bone hydroxyapatite (CBHA) has been obtained from tuna fish bone in which the carbon derived from the organics inside the bones acts as a dispersant. The XRD and TEM results indicated that the obtained HA is on the nanoscale and the N₂ adsorption/desorption isotherm showed that CBHA has mesoporous structure with an enhanced specific surface area (1129.0 m2 g?1). Moreover, CBHA as an adsorbent for removal of Congo red (CR) from aqueous solution exhibited high adsorption capacity (329.0 mg g?1) and the adsorption pattern fitted well with Langmuir model (R2 > 0.96). The adsorption kinetics of CBHA for CR followed the pseudo-second-order model. Thermodynamic parameters, including the Gibbs free energy (ΔG), enthalpy (ΔH), and entropy (ΔS), indicated that the adsorption of CR onto CBHA was feasible, spontaneous, and endothermic at the temperature range of 303–323 K. Thus, CBHA as an efficient and low-cost adsorbent can be applied to the treatment of industrial effluents contaminated with CR.

机译：含碳的骨羟基磷灰石（CBHA）是从金枪鱼鱼骨中获得的，其中来源于骨内部有机物的碳充当分散剂。 XRD和TEM结果表明，所获得的HA处于纳米级，N _{2 吸附/解吸等温线表明CBHA具有介孔结构，比表面积增加（1129.0） m 2 g ？1 ）。此外，CBHA作为用于从水溶液中去除刚果红（CR）的吸附剂具有高吸附容量（329.0 mg g ？1 ），并且吸附模式与Langmuir吻合得很好。模型（ R 2 G ），焓（Δ H ）和熵（Δ S ），表明在303–323 K的温度范围内将CR吸附到CBHA上是可行的，自发的并且是吸热的。因此，CBHA作为一种高效且低成本的吸附剂可以用于处理受CR污染的工业废水。} 展开▼

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《RSC Advances》 |2017年第43期|共6页

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Qifan Peng; Fan Yu; Bicheng Huang; Yaqin Huang;
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中图分类化学;

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1. Carbon-containing bone hydroxyapatite obtained from tuna fish bone with high adsorption performance for Congo red [J] . Peng Qifan, Yu Fan, Huang Bicheng, RSC Advances . 2017,第43期

机译：含碳骨羟基磷灰石，从金枪鱼骨中获得，具有高吸附性能的刚果红色

2. Extraction of Biological Hydroxyapatite from Tuna Fish Bone for Biomedical Applications [J] . A.F.A. LATIF, N.A.S. MOHD PUAD, N.A.A. RAMLI, Materials science forum . 2020,第1期

机译：从金枪鱼骨萃取生物羟基磷灰石，进行生物医学应用

3. Extraction of Hydroxyapatite from Fish Bones and Its Application in Nickel Adsorption [J] . Seyed Mohammad Hossein Dabiri, Amir Ardalan Rezaie, Mehrnaz Moghimi, BioNanoscience . 2018,第3期

机译：从鱼骨中提取羟基磷灰石及其在镍吸附中的应用

4. Adsorption and Removal of Zinc (II) from Aqueous Solution Using Powdered Fish Bones [C] . Han Khim Lim, Tjoon Tow Teng, Mahamad Hakimi Ibrahim International Conference on Environmental Science and Development . 2012

机译：使用粉状鱼骨料从水溶液中吸附和除去锌（II）

5. Cation and oxyanion metal sorption by iron-modified fish bone: Evaluation of a novel method to super-clean and surface-functionalize fish bone derived hydroxyapatite. [D] . Fisher, Brian D. 2012

机译：铁改性鱼骨对阳离子和氧阴离子金属的吸附：评价超清洁和表面功能化鱼骨衍生的羟基磷灰石的新方法。

6. Effects of atomic-level nano-structured hydroxyapatite on adsorption of bone morphogenetic protein-7 and its derived peptide by computer simulation [O] . Qun Wang, Menghao Wang, Xiong Lu, -1

机译：原子级纳米羟基磷灰石对骨形态发生蛋白7及其衍生肽的吸附作用的计算机模拟

7. Carbon-containing bone hydroxyapatite obtained from tuna fish bone with high adsorption performance for Congo red [O] . Qifan Peng, Fan Yu, Bicheng Huang, 2017

机译：含碳骨羟基磷灰石，从金枪鱼骨中获得，具有高吸附性能的刚果红色

8. Histological Study on a Novel Bone Graft Substitute: Human Derived Tooth-Hydroxyapatite Compared With Coralline Hydroxyapatite. [R] . Oktar, F. N., Sayrak, H., Oezsoy, S., 2001

机译：新型骨移植替代物的组织学研究：人源性牙羟基磷灰石与珊瑚羟基磷灰石的比较。

1. 碳羟基磷灰石对模拟刚果红染料废水吸附性能的研究 [J] . 王瑜 ,孙鹏跃 ,种昀楠 . 化学研究与应用 . 2020,第004期

2. 高吸附、高稳定性纳米羟基磷灰石的制备及其吸附性能研究 [J] . 郭亚丹 ,邱丽丽 ,倪悦然 . 东华理工大学学报（自然科学版） . 2015,第004期

3. 含碳酸盐氟羟磷灰石与羟基磷灰石对牛血清蛋白吸附特性的研究 [J] . 刘静 ,方玉 ,母瑞虹 . 北京口腔医学 . 2002,第003期

4. 蔗渣基吸附剂的制备及对刚果红的吸附性能 [J] . 岳新霞 ,俸海凤 ,林海涛 . 广西工学院学报 . 2017,第002期

5. 蔗渣基吸附剂的制备及对刚果红的吸附性能 [J] . 岳新霞123 ,俸海凤1 ,林海涛123 . 广西科技大学学报 . 2017,第002期

6. 三维打印羟基磷灰石/磷酸三钙骨支架工艺中粉体材料组分比及黏结剂对骨支架性能的影响 [C] . YANG Mingming ,杨明明 ,WANG Yanen . 2017江苏省先进材料研究生学术创新论坛——生物材料分论坛 . 2017

7. 羟基磷灰石与炭复合材料对水溶液中刚果红的吸附研究 [A] . 张雪祯 . 2017

1. 在用于组织和骨的支架中获得梯度孔结构的方法以及具有梯度孔结构的用于组织和骨的支架 [P] . 中国专利： CN100574817C . 2009.12.30

2. 在用于组织和骨的支架中获得梯度孔结构的方法以及具有梯度孔结构的用于组织和骨的支架 [P] . 中国专利： CN1956743A . 2007-05-02

3. a method for preparing a porcine bone graft with an excellent performance in cell adhesion and bone formation using nano hydroxyapatite surface modification technology and a porcine bone graft prepared thereby [P] . 外国专利： KR101574646B1 . 2015-12-04

机译：纳米羟基磷灰石表面改性技术制备具有良好的细胞粘附和骨形成性能的猪骨移植物的方法及由此制备的猪骨移植物

4. A METHOD FOR PREPARING A PORCINE BONE GRAFT WITH AN EXCELLENT PERFORMANCE IN CELL ADHESION AND BONE FORMATION USING NANO HYDROXYAPATITE SURFACE MODIFICATION TECHNOLOGY, AND A PORCINE BONE GRAFT PREPARED THEREBY [P] . 外国专利： KR20150125298A . 2015-11-09

机译：利用纳米羟基磷灰石表面改性技术制备具有优异细胞粘附和骨形成性能的猪骨移植物的方法及其制备的猪骨移植物

5. THE PRESENT INVENTION RELATES TO A BONE SUBSTITUTE COMPRISING A CORE BASED ON HYDROXYAPATITE (HA), OBTAINED FROM AT LEAST ONE POROUS WOOD, OR BASED ON COLLAGEN FIBRES AND HYDROXYAPATITE, AND A SHELL, BASED ON HYDROXYAPATITE (HA) OR SILICON CARBIDE (SIC), OBTAINED FROM AT LEAST ONE WOOD HAVING A LOWER POROSITY THAN THE AT LEAST ONE WOOD OF THE CORE. THE POROUS WOOD HAS A TOTAL POROSITY OF BETWEEN 60 AND 95, PREFERABLY BETWEEN 65 AND 85, AND IT IS SELECTED FROM AMONGST THE CHOICES OF RATTAN, PINE, ABACHI AND BALSA WOOD. THE WOOD OF THE SHELL HAS A POROSITY OF BETWEEN 20 AND 60, PREFERABLY BETWEEN 30 AND 50. THE BONE SUBSTITUTE IS UTILIZED FOR THE SUBSTITUTION AND REGENERATION OF BONE, PREFERABLY FOR BONES SUBJECTED TO MECHANICAL LOADS, SUCH AS LONG BONES OF THE LEG AND ARM, PREFERABLY THE TIBIA, METATARSUS, FEMUR, HUMERUS OR RADIUS. [P] . 外国专利： WO2012063201A1 . 2012-05-18

机译：本发明涉及包含基于羟基磷灰石（HA）的核心的骨替代物，所述核心取自至少一种多孔木材，或者基于胶原纤维和羟基磷灰石，以及基于羟基磷灰石（HA）的壳，是从至少一木材获得的，其孔隙率比核心的至少一木材低。多孔木材的总孔隙率在60％和95％之间，最好在65％和85％之间，并且可以从藤，松木，ABACHI和BALSA木材中选择。外壳的木材的孔隙率在20％和60％之间，最好在30％和50％之间。骨骼替代物可用于骨骼的替代和再生，尤其适用于承受机械载荷的骨骼，例如腿和手臂的长骨，通常是胫骨，变角肌，股骨，肱骨或RADIUS。

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Carbon-containing bone hydroxyapatite obtained from tuna fish bone with high adsorption performance for Congo red

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