Chiral information harvesting in helical poly(acetylene) derivatives using oligo(p-phenyleneethynylene)s as spacers

Zulema Fernández; Berta Fernández; Emilio Qui?oá; Ricardo Riguera; Félix Freire

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Chiral information harvesting in helical poly(acetylene) derivatives using oligo(p-phenyleneethynylene)s as spacers

机译：使用寡聚（对亚苯基乙烯）作为间隔物的螺旋聚（乙炔）衍生物中收获的手性信息

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A chiral harvesting transmission mechanism is described in poly(acetylene)s bearing oligo( p -phenyleneethynylene)s (OPEs) used as rigid achiral spacers and derivatized with chiral pendant groups. The chiral moieties induce a positive or negative tilting degree in the stacking of OPE units along the polymer structure, which is further harvested by the polyene backbone adopting either a P or M helix.

机译：在聚（乙炔）S轴承寡核苷酸（丙烯基乙烯）S（Opes）中描述了一种手性收割传动机制，其用作刚性成型垫片，并用手性侧基衍生化。手性部分在沿聚合物结构堆叠OPE单元的堆叠中诱导正或负倾斜程度，该聚合物结构进一步收获，该聚烯骨架采用P或M螺旋。

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《Chemical science》 |2020年第27期|共6页
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Zulema Fernández; Berta Fernández; Emilio Qui?oá; Ricardo Riguera; Félix Freire;
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1. Chiral poly(L-lactic acid) driven helical self-assembly of oligo(p-phenylenevinylene) [J] . S. Kumari Nisha, S. K. Asha Journal of Materials Chemistry, C. materials for optical and electronic devices . 2014,第11期

机译：手性聚（L-乳酸）驱动的低聚对苯撑亚乙烯基的螺旋自组装
2. Helicity Control of π-Stacked Assemblies of Oligo(para-phenylene) Derivatives Using Photoresponsive Chiral Moieties at Terminal Sites [J] . Benedict A. San Jose, Tomoki Ashibe, Naoki TActa, Advanced Functional Materials . 2014,第39期

机译：在末端位点使用光响应性手性部分控制寡聚（对亚苯基）衍生物的π堆积组装体的螺旋度
3. Synthesis of stable and soluble one-handed helical poly(substituted acetylene)s without chiral pendant groups via polymer reaction in membrane state [J] . Abe Y., Aoki T., Jia H., Polymer: The International Journal for the Science and Technology of Polymers . 2012,第11期

机译：通过膜状态下的聚合物反应合成没有手性侧基的稳定可溶的单手螺旋聚（取代乙炔）
4. Induction of One-handed Helical Oligo(p-Benzamide)s by Domino Effect Based on Planar-Axial-Helical Chirality Relay [C] . Ken Kamikawa, Keisuke Fukumoto, Kohei Yoshihara Symposium on Organometallic Chemistry . 2006

机译：基于平面轴向螺旋手足式继电器的多米诺效应诱导单手螺旋寡核苷酸（p-苯甲酰胺）S.
5. I. Tunable luminescence in dendronized poly(phenyleneethynylene)s through post-polymerization chemical modification, II. Rigid, helical polymers based upon chiral hydrobenzoin [D] . Sisk, David T. 2007

机译：I.通过后聚合化学修饰在树枝状聚（亚苯基乙炔基）中的可调发光，II。基于手性氢安息香素的刚性螺旋聚合物
6. Chiral information harvesting in helical poly(acetylene) derivatives using oligo(p-phenyleneethynylene)s as spacers [O] . Zulema Fernández, Berta Fernández, Emilio Quiñoá, 2020

机译：使用寡聚（对亚苯基乙烯）作为间隔物的螺旋聚（乙炔）衍生物中收获的手性信息
7. Chiral information harvesting in helical poly(acetylene) derivatives using oligo(p-phenyleneethynylene)s as spacers [O] . Zulema Fernández, Berta Fernández, Emilio Quiñoá, 2020

机译：使用寡聚（对亚苯基乙烯）作为间隔物的螺旋聚（乙炔）衍生物中收获的手性信息
8. Thermoset Polymers Made by Blending Poly (Carborane-Siloxane/ Silane-Acetylene)and Poly (Siloxane/Silane-Acetylene) [R] . Keller, T. M., Son, D. Y. 1996

机译：通过混合聚（碳硼烷 - 硅氧烷/硅烷 - 乙炔）和聚（硅氧烷/硅烷 - 乙炔）制成的热固性聚合物

Chiral information harvesting in helical poly(acetylene) derivatives using oligo(p-phenyleneethynylene)s as spacers

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