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首页> 外文期刊>Communications Physics >High efficiency ultrafast water-window harmonic generation for single-shot soft X-ray spectroscopy
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High efficiency ultrafast water-window harmonic generation for single-shot soft X-ray spectroscopy

机译:高效超快水窗谐波生成单次软X射线光谱

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Fully coherent, soft X-ray attosecond pulses are now available through high-order harmonic generation (HHG); however, the output energy is insufficient for various applications, such as attosecond-scale soft X-ray nonlinear experiments, the seeding of soft X-ray free-electron lasers, attosecond-pump-attosecond-probe spectroscopies, and single-shot imaging. In this paper, we combine a newly developed TW class mid-infrared femtosecond laser and a loose focusing geometry for HHG. A soft X-ray harmonic beam up to the water window region is demonstrated, which is more than 100 times intense compared to previous works. We achieve a high conversion efficiency, low beam divergence and a significantly reduced medium gas pressure. As the first application, we demonstrate near edge X-ray absorption fine structure experiments with clear fine absorption spectra near the K- and L-edges observed. The robust energy scaling method on HHG opens the door for demonstrating single-shot absorption spectrum and live-cell imaging with a femtosecond time resolution. While high harmonic x-ray sources are well established sources for ultrafast spectroscopy, the decrease in efficiency towards higher energies limits their application. Here, a loose-focused, TW mid-IR laser is used to generate high harmonic soft x-rays with pulse energies of a few nJ in the water window and easy energy scaling.
机译:完全相干,软X射线抗折叠脉冲现在可通过高阶谐波发电(HHG)提供;然而,输出能量对于各种应用不足,例如抗秒级软X射线非线性实验,软X射线自由电子激光器的播种,AttoSecond-Pump-Attosecond-探针光谱和单次成像。在本文中,我们将新开发的TW类中红外飞秒激光器和HHG的松散聚焦几何相结合。对水窗区域的柔软X射线谐波横梁进行了说明,与之前的作品相比大于100倍。我们达到了高转换效率,低光束发散和显着降低的介质气体压力。作为第一个申请,我们展示了近边缘X射线吸收细结构实验,在观察到的K-和L边缘附近具有清晰的精细吸收光谱。 HHG上的鲁棒能量缩放方法打开门,用于展示单次吸收光谱和具有飞秒时间分辨率的活细胞成像。虽然高谐波X射线源是超快速光谱的很好的源,但较高能量效率的降低限制了它们的应用。这里,可轻松聚焦的TW Mid-IR激光器用于产生高谐波软X射线,在水窗口中具有几个NJ的脉冲能量,并且易于能量缩放。

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