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Mass concentration, optical depth and carbon composition of particulate matter in the major southern West African cities of Cotonou (Benin) and Abidjan (C?te d'Ivoire)

机译:Cotonou(贝宁)和Abidjan的主要南部西非城市颗粒物质的质量浓度,光学深度和碳成分(C?TE D'IVOIRE)

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Air quality degradation is a?major issue in the large conurbations on the shore of the Gulf of Guinea. We present for the first time PM2.5 time series collected in Cotonou, Benin, and Abidjan, C?te d'Ivoire, from February?2015 to March?2017. Measurements were performed in the vicinity of major combustion aerosol sources: Cotonou/traffic (CT), Abidjan/traffic (AT), Abidjan/landfill (AL) and Abidjan/domestic fires (ADF). We report the weekly PM2.5 mass and carbonaceous content as elemental (EC) and organic (OC) carbon concentrations. We also measure the aerosol optical depth (AOD) and the ?ngstr?m exponent in both cities. The average PM2.5 mass concentrations were 32±32, 32±24 and 28±19μg?m?3 at traffic sites CT and AT and landfill site AL, respectively. The domestic fire site shows a concentration of 145±69μg?m?3 due to the contribution of smoking and roasting activities. The highest OC and EC concentrations were also measured at ADF at 71±29 and 15±9μg?m?3, respectively, while the other sites present OC concentration between 8 and 12μg?m?3 and EC concentrations between 2 and 7μg?m?3. The OC∕EC ratio is 4.3 at CT and 2.0 at AT. This difference highlights the influence of two-wheel vehicles using gasoline in Cotonou compared to that of four-wheel vehicles using diesel fuel in Abidjan. AOD was rather similar in both cities, with a?mean value of 0.58 in Cotonou and of 0.68 in Abidjan. The seasonal cycle is dominated by the large increase in surface mass concentration and AOD during the long dry season (December–February) as expected due to mineral dust advection and biomass burning activities. The lowest concentrations are observed during the short dry season (August–September) due to an increase in surface wind speed leading to a?better ventilation. On the other hand, the high PM2.5∕AOD ratio in the short wet season (October–November) indicates the stagnation of local pollution.
机译:空气质量退化是一个?几内亚海湾岸边的大型电都的主要问题。我们首次出现PM2.5时间系列在Cotonou,Benin和Abidjan,C?Te D'Ivoire,从2月到2015年到3月?2017年。测量是在主要燃烧气溶胶源附近进行的:Cotonou /交通(CT),Abidjan /交通(AT),Abidjan /垃圾填埋场(AL)和Abidjan /家庭火灾(ADF)。我们将每周PM2.5质量和碳质含量报告为元素(EC)和有机(OC)碳浓度。我们还测量了两个城市的气溶胶光学深度(AOD)和?NGSTR?M指数。平均PM2.5质量浓度分别在交通站点CT和AT和垃圾填埋场AL下分别为32±32,22,24和28±19μg≤3.3。由于吸烟和烘焙活动的贡献,国内火灾部位显示出145±69μg的浓度为145±69μg?3。在ADF的ADF下分别在71±29和15±9μg≤M≤3,而另一种位点在8至12μg≤M≤3和2至7μg的EC浓度下,分别在71±29和15±9μgΩ·m?3处测量最高的OC和EC浓度。 ?3。在CT和2.0时,OC / EC比率为4.3。与阿比哈丹柴油燃料的四轮车辆相比,这种差异突出了双轮车辆在Cotonou中使用汽油的影响。 AOD在两个城市中相当相似​​,Cotonou的平均值为0.58,Abidjan为0.68。由于矿物粉尘平流和生物质燃烧活动,季节性循环在长旱季(12月至2月)期间的表面质量浓度和AOD的大幅增加。由于表面风速的增加导致通风更好,在短旱季(八月至9月)期间观察到最低浓度。另一方面,短暂的PM2.5 / AOD比率在短暂的潮湿季节(十月至11月)表示局部污染的停滞。
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