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Atmospheric new particle formation: real and apparent growth of neutral and charged particles

机译:大气新的粒子形成:中性和带电粒子的真实和明显的生长

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In this study we have provided simple analytical formulae to estimate the growth rate of a nucleation mode due to self-coagulation and the apparent growth rate due to coagulation scavenging by larger particles. These formulae were used on a set of simulations covering a wide range of atmospheric conditions. The modal growth rates were determined from the simulation results by summing the contribution of each process, by calculating the increase rate in the count mean diameter of the mode and by following the peak concentration of the mode. The results of these three methods were compared with each other and the means used to estimate the growth rate due to self-coagulation and coagulation scavenging were found to give accurate values. We also investigated the role of charged particles and electric interactions in the growth of a nucleation mode. Charged particles were found to increase the growth rate due to both self-coagulation and coagulation scavenging by a factor of ~1.5 to 2. In case of increased condensation onto charged particles, the total condensational growth rate of a nucleation mode may increase significantly in the very early steps of the growth. The analytical formulae provided by this paper were designed to provide the growth rates due to different processes from aerosol dynamic simulations, but the same principles can be used to determine the growth rates from measurement data.
机译:在该研究中,我们提供了简单的分析公式,以估计由于自凝固而导致的成核模式的生长速率和由于较大的颗粒清除凝固而具有表观生长速率。这些配方用于覆盖各种大气条件的一组模拟。通过计算模式的计数平均直径的增加率并通过遵循模式的峰值浓度来从模拟结果求解模拟结果,从模拟结果中确定模拟结果。认为这三种方法的结果彼此进行比较,并且发现用于估计由于自凝固和凝固清除引起的生长速率的手段得到了准确的值。我们还研究了带电粒子和电相互作用在成核模式的生长中的作用。发现带电粒子由于自凝固和凝固而凝结的凝固术增加了〜1.5至2.在带电粒子上的缩合增加的情况下,成核模式的总致敏生长速率可能会显着增加这一增长的早期步骤。本文提供的分析公式旨在提供由于气溶胶动态仿真的不同过程,而且可以使用相同的原理来确定来自测量数据的生长速率。

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