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Interactions of Single Particle with Organic Matters: A Facile Bottom-Up Approach to Low Dimensional Nanostructures

机译：单粒子与有机物质的相互作用：低尺寸纳米结构的容易自下而上的方法

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A particle induces a pack of chemical reactions in nanospace: chemical reactions confined into extremely small space provide an ultimate technique for the nanofabrication of organic matter with a variety of functions. Since the discovery of particle accelerators, an extremely high energy density can be deposited, even by a single isolated particle with MeV-ordered kinetic energy. However, this was considered to cause severe damages to organic molecules due to its relatively small bond energies, and lack of ability to control the reactions precisely to form the structures while retaining physico-chemical molecular functionalities. Practically, the severely damaged area along a particle trajectory: a core of a particle track has been simply visualized for the detection/dosimetry of an incident particle to the matters, or been removed to lead nanopores and functionalized by refilling/grafting of fresh organic/inorganic materials. The use of intra-track reactions in the so-called “penumbra” or “halo” area of functional organic materials has been realized and provided us with novel and facile protocols to provide low dimensional nano-materials with perfect size controllability in the 21st century. These protocols are now referred to as single particle nanofabrication technique (SPNT) and/or single particle triggered linear polymerization technique (STLiP), paving the way towards a new approach for nanomaterials with desired functionalities from original molecules. Herein, we report on the extremely wide applicability of SPNT/STLiP protocols for the future development of materials for opto-electronic, catalytic, and biological applications among others.
机译：颗粒在纳米周中诱导一包化学反应：局限于极小空间的化学反应提供了具有多种功能的有机质纳米制剂的最终技术。由于颗粒促进剂的发现，甚至可以沉积极高的能量密度，甚至可以沉积极高的能量密度，甚至可以通过具有透射lev订购的动能的单个分离的颗粒。然而，这被认为由于其相对较小的粘合能而导致有机分子对有机分子产生严重损伤，并且缺乏控制反应的能力，该能力精确地形成结构，同时保持物理化学分子功能。实际上，沿粒子轨迹的严重受损区域：粒子轨道的核心已经简单地被视为入射颗粒的检测/剂量，或者被除去以引导纳米孔并通过重新填充/嫁接新鲜有机/脱气无机材料。已经实现了在所谓的“PENUMBRA”或“光环”区域中的轨道内反应已经实现了功能性有机材料的区域，并为我们提供了新颖的和容易方案，以提供21世纪具有完美尺寸可控性的低维纳米材料。这些方案现在被称为单粒子纳米制作技术（SPNT）和/或单粒子触发的线性聚合技术（STLIP），铺平了从原始分子的所需功能的纳米材料的新方法。在此，我们报告了SPNT / STLIP协议的极广泛适用性，用于未来的光电，催化和生物应用的材料的未来发展。

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